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Association of gut microbiota and immunometabolic profiles with ischemic stroke severity

Scientific Reports Claudio Roberto Scolari Pilon, Dioze Guadagnini, Heloisa B. Assalin et al. Apr 23, 2025 DOI: 10.1038/s41598-025-97432-2

Involving Carbene or Not? Mechanism of Corey–Winter Reaction

Journal of the American Chemical Society Pan Zhang, Zhi-Xiang Yu Apr 23, 2025 DOI: 10.1021/jacs.5c02629

Development of manganese ferrite coated with Prussian blue as an efficient contrast agent for applications in magnetic resonance imaging

Scientific Reports Ágnes Mária Ilosvai, Fatemeh Heydari, László Forgách et al. Apr 23, 2025 DOI: 10.1038/s41598-025-98348-7

Abstract Magnetic iron oxide nanoparticles are frequently utilized as contrast agents in magnetic resonance imaging (MRI). However, the release of iron ions leads to the formation of reactive oxygen species (ROS), resulting in cell damage. In this study, we developed MRI contrast agents containing amine-functionalized MnFe2O4 nanoparticles with a Prussian blue (PB) surface coating to enhance their biocompatibility. The prepared MNPs were embedded in polyvinylpyrrolidone and dried. The resulting crystals can be redispersed in water immediately before use, forming a stable colloid. The particle size of nanoparticles (43 ± 13 nm) is suitable for the intended application. The values of Hc (52 Oe) and Mr (3.7 emu/g) for the particles indicate a soft ferromagnetic nature. The coating of the particles with PB results in a significant reduction of their toxicity, as evidenced by a toxicological test on HEK293 cells. This colloid was tested in vitro as an MRI contrast agent as well as in healthy animal. The longitudinal relaxivity (r1) of the PB-MnFe2O4-NH2 sample was determined to be 0.01 (mg/mL)−1ms− 1. The transversal relaxivity was measured as well (r2: 0.77 (mg/mL)−1ms− 1 and r2*: 1.48 (mg/mL)−1ms− 1, which were in the same range as Feraheme and Endorem. Prussian blue-coated MnFe2O4 emerges as a promising T2-weighted contrast material, representing a novel combination of two well-known contrast-capable materials.

Cyclic Bifunctional Reagents Enabling a Strain-Release-Driven Formal [3 + 2] Cycloaddition of 2<i>H</i>-Azirines by Cascade Energy Transfer

Journal of the American Chemical Society Alessia Petti, Mathis J. Karrasch, Preeti Chahar et al. Apr 23, 2025 DOI: 10.1021/jacs.4c18080

Open-circuit diagnosis method based on dual-mode voltage residual model for T-type three-level inverter

Scientific Reports Liming Song, Minxuan Liao, Rongkun Wang et al. Apr 23, 2025 DOI: 10.1038/s41598-025-98747-w

Abstract This study proposes a rapid online diagnostic method based on a dual-mode line voltage residual model for diagnosing IGBT open-circuit faults in a T-type three-level inverter. The method is based on the voltage residual method and is integrated with a three-level fault-tolerant algorithm. Firstly, by analyzing the line voltage residuals after an open-circuit fault in the T-type inverter under normal operating conditions, 12 types of single-switch open-circuit faults are divided into 6 groups. Next, the breakdown of the spatial voltage vectors following the fault are analyzed, and the remaining vectors are reconfigured to enable the inverter’s operation under three-level fault-tolerant control. In the fault-tolerant control, the residual voltage returns to its normal value, aiding in precise fault localization. Simulation and experimental results validate the method’s robustness against load variations. This method significantly increases diagnostic speed and reduces harmonic interference in the diagnosis procedure. These findings are of paramount importance for fault diagnosis and the reliable operation of the T-type three-level inverter.

Rational Design of PROTAC Linkers Featuring Ferrocene as a Molecular Hinge to Enable Dynamic Conformational Changes

Journal of the American Chemical Society Alessandra Salerno, Lianne H. E. Wieske, Claudia J. Diehl et al. Apr 23, 2025 DOI: 10.1021/jacs.4c18354

Critical success factors for successful technology innovation development in sustainable energy enterprises

Scientific Reports T. A. Alka, Raghu Raman, M. Suresh Apr 23, 2025 DOI: 10.1038/s41598-025-98725-2

Regiodivergent Hydroamidation of Alkenes via Cobalt-Hydride Catalysis

Journal of the American Chemical Society Bingxue Liu, Qianqian Lu, Xiao Hu et al. Apr 23, 2025 DOI: 10.1021/jacs.5c03484

First record of a living coelacanth from North Maluku, Indonesia

Scientific Reports Alexis Chappuis, I Gede Hendrawan, M. Janib Achmad et al. Apr 23, 2025 DOI: 10.1038/s41598-025-90287-7

Regulating Enol-to-Keto Tautomerization of Pillararene-Based Conjugated Macrocycle Polymers for H<sub>2</sub>O<sub>2</sub> Photosynthesis

Journal of the American Chemical Society Zhuo-Qin Wang, Meng-Hao Li, Shuang Liang et al. Apr 23, 2025 DOI: 10.1021/jacs.5c00768

Family structure factors influencing modern contraceptive use in Cameroon based on analysis of 2018–2019 demographic and health survey data

Scientific Reports Samira Amadou, Myungken Lee, Jakyoung Lee et al. Apr 23, 2025 DOI: 10.1038/s41598-025-85998-w

Rapid Access to Small Molecule Conformational Ensembles in Organic Solvents Enabled by Graph Neural Network-Based Implicit Solvent Model

Journal of the American Chemical Society Paul Katzberger, Lea M. Hauswirth, Antonia S. Kuhn et al. Apr 23, 2025 DOI: 10.1021/jacs.4c17622

Epidemiological and spatiotemporal analysis of elderly HIV-1/AIDS patients in Ningxia, China, from 2018 to 2023

Scientific Reports Zhonglan Wu, Yichang Liu, Xiaofa Ma et al. Apr 23, 2025 DOI: 10.1038/s41598-025-98791-6

Abstract To analyze the epidemiological transmission characteristics and spatiotemporal distribution patterns of the elderly HIV-1/AIDS population in NHAR from 2018 to 2023, to provide theoretical support for the targeted formulation and implementation of HIV-1 interventions. A cross-sectional study was conducted in August 2024. Plasma samples were collected from the elderly HIV-1/AIDS patients (&gt; 50 years old) in NHAR, followed by RNA extraction and RT-PCR to amplify the pol gene of HIV-1. The amplicons were sequenced for the partial pol region. Subtyping was performed using online tools from the HIV-1 database and MEGA11. Drug resistance was analyzed using the Stanford University HIVdb algorithm. Molecular transmission networks were constructed using Cytoscape 3.10.0. Logistic regression was performed to identify the potential risk factors. Spatial analysis revealed the geographic patterns of elderly HIV-1/AIDS patients. A total of 208 HIV-1/AIDS patients were included in this study, predominantly male (78.37%), primary school and below (46.63%), heterosexual transmission (80.77%) and farmers (52.40%). Nine genetic subtypes were identified, with CRF07_BC being the most common (54.81%). The overall drug resistance rate was 37.98%. The number of network nodes increased from 18 in 2018 to 107 in 2023, with large propagating clusters in 2023 merging or expanding from smaller clusters in previous years. Logistic regression analysis showed that males had a lower risk of transmission, individuals from Yinchuan, Shizuishan, and Wuzhong had a lower probability of entering the network, and CRF07_BC and CRF01_AE had a higher risk of transmission. From 2020 to 2023, there was a highly significant clustering pattern among elderly HIV/AIDS patients in NHAR, with shifts in hotspots. Yuanzhou District remained a persistent cold spot. This study reveals that the elderly HIV-1/AIDS patients in NHAR were predominantly married, male, and engaged in farming, with low levels of education. An increase in the diversity of viral genetic subtypes was observed, along with a high rate of drug resistance. The molecular network expanded significantly, accompanied by the emergence of large transmission clusters, indicating complex transmission patterns. The spatial distribution of these cases exhibited aggregation, with notable differences observed between districts and counties. To effectively intervene in the transmission of HIV-1 among the elderly population, it is essential to establish a long-term dynamic molecular transmission surveillance network and to improve AIDS screening and drug resistance testing.

Local Ionic Conditions Modulate the Aggregation Propensity and Influence the Structural Polymorphism of α-Synuclein

Journal of the American Chemical Society Maria Zacharopoulou, Neeleema Seetaloo, James Ross et al. Apr 23, 2025 DOI: 10.1021/jacs.4c13473

Enhancing tuberculosis (TB) case detection among hospitalized patients through lay health worker led screening: a before-and-after study in KwaZulu-Natal, South Africa

Scientific Reports Abera Balcha Bulti, Asnake Yohannes Dumicho, Altynay Shigayeva et al. Apr 23, 2025 DOI: 10.1038/s41598-025-90497-z

Porphyrin-Engineered <sup>125</sup>I-Nanoseeds as a Prototype for Immunogenic Brachytherapy

Journal of the American Chemical Society Zhiyu Tu, Ziyang Sang, Yang Xu et al. Apr 23, 2025 DOI: 10.1021/jacs.4c17573

Peritumoral features for assessing invasiveness of lung adenocarcinoma manifesting as ground-glass nodules

Scientific Reports Xiao Wang, Hui Xue, Wei Ding et al. Apr 23, 2025 DOI: 10.1038/s41598-025-99180-9

Cyclometallated Co(III) Complexes with Lowest-Energy Charge Transfer Excited States Accessible with Visible Light

Journal of the American Chemical Society Spencer T. Burton, Gyunhee Lee, Curtis E. Moore et al. Apr 23, 2025 DOI: 10.1021/jacs.4c18299

Author Correction: Enhancing the power quality of dual rotor wind turbines using improved fuzzy space vector modulation and super twisting sliding techniques

Scientific Reports Habib Benbouhenni, Nicu Bizon, Mourad Yessef et al. Apr 23, 2025 DOI: 10.1038/s41598-025-99359-0

Correction to “In Situ Probing the Anion-Widened Anodic Electric Double Layer for Enhanced Faradaic Efficiency of Chlorine-Involved Reactions”

Journal of the American Chemical Society Mingming Yan, Rong Yang, Cuibo Liu et al. Apr 23, 2025 DOI: 10.1021/jacs.5c05221