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Shallow Hole Trapping and Intrinsic Defect Tolerance in Visible-Light Photocatalysts: The Role of Lattice Relaxation and Electronic Screening

Journal of the American Chemical Society Akira Yamakata, Junie Jhon M. Vequizo, Kazunari Domen Apr 22, 2026 DOI: 10.1021/jacs.6c00026

Multi-session smart night charging of EVs for accelerated decarbonization of electric mobility

PLoS ONE Felix Wieberneit, Emanuele Crisostomi, Anthony Quinn et al. Apr 22, 2026 DOI: 10.1371/journal.pone.0345748

The majority of electric vehicles (EVs) are charged domestically overnight, when the precise timing of power allocation is not important to the user, thus providing a source of flexibility that can be leveraged by charging control algorithms. In this paper, we show that by keeping the EV connected to a standard domestic smart plug every night, it is possible to achieve an approximate 37% annual reduction in carbon intensity compared to uncontrolled charging (based on 2022 UK National Grid data) without compromising the EV owners’ charging demand. For this purpose, we use Model Predictive Control techniques to schedule power delivery with the objective of minimizing grid-average CO 2 emissions over forecast windows of multiple sessions (up to seven days ahead). We find that flexibility on the part of EV owners—both their willingness to keep the EV connected at night, and to indicate a precautionary (i.e., upper bound) estimate of their required state-of-charge in the morning—allows for significant emissions reduction and accelerated decarbonization of the mobility sector.

Alkyne Cyclizations through Vinyl Cations and Stereoselective Allene Formation by Terpene Synthases

Journal of the American Chemical Society Alain C. Tumma, Houchao Xu, Bernd Goldfuss et al. Apr 22, 2026 DOI: 10.1021/jacs.6c05306

Editorial Note: Cohort profile: The Endometriosis pain QUality aftEr Surgical Treatment (EndoQUEST) Study

PLoS ONE Apr 22, 2026 DOI: 10.1371/journal.pone.0347712

Gas-Phase and Condensed-Phase Synergy in a Nonflammable Electrolyte for Highly Stable Sodium-Ion Batteries

Journal of the American Chemical Society Wensha Niu, Peng-Tao Guo, Meng-Nuo Wu et al. Apr 22, 2026 DOI: 10.1021/jacs.6c05618

Exploring the key points and key shots in table tennis matches based on survival analysis

PLoS ONE Muzi Li, Qing Yang Apr 22, 2026 DOI: 10.1371/journal.pone.0338203

This study aimed to investigate the Key Points ( KP ) and Key Shots ( KS ) in singles matches for elite table tennis players, enhancing the knowledge of winning patterns in table tennis. A total of 60 men’s singles and 64 women’s singles matches were analyzed, all data sourced from events such as the World Championships, World Cup, Olympic Games, and WTT Champions. Methods: Survival analysis was introduced, in which points scored in a match and shot counts in a rally were treated as “survival time,” while losing a point was defined as the “event.” The Kaplan-Meier method was employed to estimate cumulative survival probabilities, which reflect the likelihood of players enhancing their winning potential at specific scores or shot numbers. The point or shot number at which the cumulative survival probability drops to 50% is defined as the KP or KS , respectively. Additionally, the Log-rank (Mantel-Cox) non-parametric test was applied to determine whether significant differences existed between the survival curves of different groups. Results: KP in table tennis singles demonstrate a stable pattern of “ 7 for women, 8 for men,” while Winning Points ( WP ) are predominantly concentrated at the 9th point. The KS positions are consistent in both men’s and women’s singles, specifically the 4th shot in the total rally, the 3rd shot in the serving round, and the 2nd shot in the receiving round. Winning Shots ( WS ) consistently occur at the 6th shot in the total rally, as well as the 3rd shot in both the serving and receiving rounds. Conclusion: These findings advance our understanding of winning patterns in table tennis, providing theoretical foundations and practical references for designing contextualized training programs, precisely regulating athletes’ competitive psychology, and optimizing future competition rules.

Dual-Targeting Multivalent Aptamer-Drug Hybrids for Synergistic Cancer Immunotherapy

Journal of the American Chemical Society Hongli Chi, Yanlin Du, Wei Lv et al. Apr 22, 2026 DOI: 10.1021/jacs.5c21968

EconoGNN: A graph neural network framework for temporal economic resilience insights

PLoS ONE Marcus Araujo, Francisco Rodrigues, Elaine Sousa Apr 22, 2026 DOI: 10.1371/journal.pone.0343683

Global economic shocks such as the 2008 financial crisis or recent trade escalations between the United States and China have exposed the complexity of interdependent economies and the need for systemic, multi-agent analysis. However, most regional economic resilience (RER) studies remain limited by localized datasets, inconsistent definitions, and static modeling approaches, restricting their ability to generalize insights across space and time. We introduce EconoGNN, a Graph Neural Network framework that integrates complexity theory, economic modeling, and machine learning to predict and explain regional economic resilience across 183 countries over 25 years. By combining over 81 million trade records (UN COMTRADE) and 500,000 macroeconomic observations (Penn World Table), and adopting an official resilience metric from the World Bank, our approach enables reproducible and interpretable global-scale analysis. EconoGNN achieves F1-scores of 0.750 with the temporal GNN architecture GConvGRU, AUC-ROC of 0.792, and PR-AUC of 0.757, demonstrating robust performance across different recovery threshold settings ( τ = 0.90–1.00) with F1-scores ranging from 0.730 to 0.771, and yielding statistically significant improvements (p-value ≤0.05) over baselines. GNNExplainer validation confirms explanation reliability (Fidelity+ = 0.827, Characterization = 0.913), enabling country-customized interpretability of resilience drivers. Moreover the EconoGNN framework integrates key structural and welfare indicators to model both national and cross-border economic interactions, reducing omitted-variable bias and implicitly accounting for political, institutional, and cultural differences.

Comprehensive analysis of immune-related genes reveals diagnostic biomarkers and molecular subtypes in diabetic retinopathy

PLoS ONE Lin Mu, Zhe Wang, Yaojiani Cao et al. Apr 22, 2026 DOI: 10.1371/journal.pone.0346725

Diabetic retinopathy (DR) is a common microvascular complication of diabetes and one of the primary causes of vision loss; however, its pathogenic mechanisms remain largely unresolved. In recent years, immune dysregulation has been increasingly recognized to be closely associated with DR progression. In the present study, we integrated two GEO datasets to identify immune-related differentially expressed genes (DEGs) associated with DR. After batch effect correction and differential expression analysis, a total of 123 immune-related DEGs were identified. Functional enrichment analysis demonstrated that these genes are primarily associated with immune activation pathways, such as T-cell receptor signaling, natural killer cell–mediated cytotoxicity, and IL-17 signaling. Using least absolute shrinkage and selection operator (LASSO) regression, five key genes (IL10RA, PLAUR, PLAU, VTN, and VGF) were identified and used to construct a diagnostic model with excellent predictive performance. Protein–protein interaction and immune infiltration analyses revealed that these genes are closely associated with immune cell activity, particularly the increased infiltration of resting CD4 memory T cells and M2 macrophages in the DR retina. To validate these findings, an STZ-induced diabetic mouse model was used, with key genes further validated at the protein level via Western blot. In addition, consensus clustering was used to stratify patients with DR into two molecular subtypes with distinct immune characteristics and pathway enrichment patterns. Overall, our study elucidates the immune-related mechanisms underlying DR and highlights PLAUR, PLAU, and VGF as potential immune-associated biomarkers, providing a theoretical basis for precision diagnosis and development of targeted immunotherapeutic strategies for DR.

Controlling Electrode–Electrolyte Interactions to Enhance Capacitance

Journal of the American Chemical Society Jamie W. Gittins, Chloe J. Balhatchet, James Hill et al. Apr 22, 2026 DOI: 10.1021/jacs.5c20988

RMETNet: A cross-subject motor imagery EEG signal classification model based on TSLANet and riemannian geometry features

PLoS ONE Yun Zhao, Dongyi He, Fudai Ren et al. Apr 22, 2026 DOI: 10.1371/journal.pone.0347671

Motor imagery electroencephalogram (MI-EEG) analysis is essential for natural interaction and autonomous control in brain-computer interfaces (BCIs). However, deep learning models often struggle with inter-subject variability, which limits their ability to generalize across subjects. This study proposes RMETNet, a novel framework that integrates TSLANet, a spatio-temporal convolution module, and a multi-scale Riemannian geometry feature module. TSLANet suppresses noise and captures complex temporal patterns for preliminary signal decoding, while the spatio-temporal convolution module extracts higher-order representations. The Riemannian branch learns geometry-based distribution features across subjects, and the fused features are used for classification. To address inter-subject distribution shifts, RMETNet incorporates Maximum Mean Discrepancy (MMD) loss for domain adaptation, aligning feature distributions between source and target domains. Experiments show that on the four-class BCI Competition IV 2a (BCICIV2a) dataset, RMETNet achieved accuracies of 71.39% in the cross-subject setting and 80.71% in the subject-dependent setting; on the two-class BCI Competition IV 2b (BCICIV2b) dataset, it achieved 80.93% and 86.76%, respectively. The model consistently outperformed baseline algorithms. Ablation and visualization analyses further validated its effectiveness in reducing inter-subject feature distribution disparities and enhancing MI-EEG decoding. The code is available at: https://github.com/rokanfeermecer486/RMETNet .

Total Synthesis of Euphopia B and Discovery of a Selective Inhibitor of Potassium Efflux-Independent NLRP3 Inflammasome Activation

Journal of the American Chemical Society Chaoyun Xue, Ze Zhang, Zhongpeng Ding et al. Apr 22, 2026 DOI: 10.1021/jacs.6c02838

A pH-Responsive Cu-Corrole-Based Cage That Reversibly Encapsulates Fullerene in a Shapeshifting Low-Symmetry Cavity

Journal of the American Chemical Society Anna Baidiuk, Tània Pèlachs, Paul-Gabriel Julliard et al. Apr 22, 2026 DOI: 10.1021/jacs.5c21440

Rational Design of High-Na P2-Type Cathodes for Sodium-Ion Batteries: Unveiling Phase Formation Principles and Composition–Structure–Performance Correlations

Journal of the American Chemical Society Yitong Zhou, Jinfang Wu, Shuyin Xu et al. Apr 22, 2026 DOI: 10.1021/jacs.5c20111

Localized Cation Unlocks Unique Activity-Selectivity Trends in Molecular Oxygen Reduction Catalysis

Journal of the American Chemical Society Hwi Yul Jo, Vom Kang, Dongyoung Kim et al. Apr 22, 2026 DOI: 10.1021/jacs.5c18246

Enantioselective Total Syntheses of Grayanoid (−)-Mollfoliagein A and (−)-Rhodomollein XXV

Journal of the American Chemical Society Shu-Fei Du, Yi-Peng Zhang, Quan-Lin Wu et al. Apr 22, 2026 DOI: 10.1021/jacs.6c03596

Rhodium-Catalyzed Desymmetric Addition of Boronic Acids to Malononitriles

Journal of the American Chemical Society Minghao Zhang, Qihao Zhang, Junjie Cao et al. Apr 22, 2026 DOI: 10.1021/jacs.5c23045

Site-Specifically Modified Circular Ribonucleic Acid Serves as Multitarget miRNA Sponge with Low Immunogenicity

Journal of the American Chemical Society Yufan Pan, Xin Li, Bini Zhou et al. Apr 22, 2026 DOI: 10.1021/jacs.6c04991

Diffusion-Mediated Synthesis of Durable High-Entropy Sulfide Nanocrystals: Le Chatelier-Driven and Electron Configuration Effects

Journal of the American Chemical Society Pengfei Da, Zhuang Zhang, Xiaoyue Qiang et al. Apr 22, 2026 DOI: 10.1021/jacs.6c02607

Iron-Catalyzed Cross-[2 + 2] Cycloaddition of Butadiene and α,ω-Dienes for Ductile and Chemically Recyclable Poly(oligocyclobutanes)

Journal of the American Chemical Society Cherish Nie, Sahana V. Sundar, Hang Zhang et al. Apr 22, 2026 DOI: 10.1021/jacs.5c23398