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The edge orientation entropy of natural scenes is associated with infant visual preferences and adult aesthetic judgements

PLoS ONE Philip McAdams, Sara Svobodova, Taysa-Ja Newman et al. Feb 26, 2025 DOI: 10.1371/journal.pone.0316555

Statistical regularities of oriented edges in natural scenes, ‘edge co-occurrence statistics’, are associated with adults’ aesthetic responses, with greater preference for some images when the degree of randomness in the orientation of edges (Edge Orientation Entropy, EOE) across an image is relatively high. Here, we investigate whether this spatial image statistic is also associated with infants’ visual preferences. We measure infant looking time for images of building façades previously used to identify the relationship between EOE and adult aesthetic judgements. Twenty-six 4–9-month-old infants and 29 adults looked freely at pairs of the images. Infants and adults both looked longest at images where all edge orientations are about equally likely to occur (high 1st-order EOE), and at images with low correlation of edge orientations across the image (high 2nd-order EOE). Infant looking time and adult pleasantness judgements were also strongly related: infants looked longer at the building façades that adults liked. Our results suggest that even as young as 4-months, infants’ spatial vision is sensitive to edge co-occurrence statistics that are typical of natural scenes and faces, where edges are more evenly distributed across orientations. We discuss the implications for understanding the sensory component of adult aesthetic judgements, as well as the role of natural scene statistics in infant perception.

Adaptive control and state error prediction of flexible manipulators using radial basis function neural network and dynamic surface control method

PLoS ONE Yang Zhang, Liang Zhao Feb 26, 2025 DOI: 10.1371/journal.pone.0318601

This paper introduces a novel control strategy for managing the uncertainties in flexible joint manipulators, incorporating a Radial Basis Function Neural Network (RBFNN) with Adaptive Dynamic Surface Control (ADSC). This strategy innovatively utilizes RBFNN to precisely approximate uncertain system dynamics and integrates a nonlinear damping term to effectively counteract external disturbances, enhancing the overall control accuracy. We have also developed an adaptive law that updates neural network weights and system parameters in real-time, ensuring the system’s adaptability to dynamic changes. The application of the Lyapunov method ensures that all signals within the closed-loop system remain semi-globally uniformly bounded, significantly reducing tracking errors. Moreover, we introduce the use of Long Short-Term Memory (LSTM) networks for predictive analysis of state data, which further confirms the robustness and effectiveness of our control method through extensive simulations. The distinctive integration of these technologies and their practical validation through comparative simulations underscore the innovative aspects of our approach in addressing real-world challenges in flexible manipulators.

One-Step HF-Free Synthesis of Alkali Metal Fluorides from Fluorspar

Journal of the American Chemical Society Thomas Schlatzer, Christopher A. Goult, Michael A. Hayward et al. Feb 26, 2025 DOI: 10.1021/jacs.4c16608

Facile Synthesis of Housanes by an Unexpected Strategy

Journal of the American Chemical Society Yanyao Liu, Somanea Tranin, Yu-Che Chang et al. Feb 26, 2025 DOI: 10.1021/jacs.4c13298

Mechanism-Based Inhibition of Histone Deacetylase 6 by a Selenocyanate Is Subject to Redox Modulation

Journal of the American Chemical Society Juana Goulart Stollmaier, Briana Abigail R. Czarnecki, David W. Christianson Feb 26, 2025 DOI: 10.1021/jacs.5c00157

Controlling Interlayer Disorder Toward Reversible Phase Transition in a Layered Sodium Manganese Oxide Cathode

Journal of the American Chemical Society Seongkoo Kang, Jihyun Kim, Youngju Choi et al. Feb 26, 2025 DOI: 10.1021/jacs.4c15913

Engineering the Lewis Acidity of Fe Single-Atom Sites via Atomic-Level Tuning of Spatial Coordination Configuration for Enhanced Oxygen Reduction

Journal of the American Chemical Society Qingyun Qu, Yu Mao, Shufang Ji et al. Feb 26, 2025 DOI: 10.1021/jacs.4c17444

Enhancing Selective Hydrofluorocarbon Greenhouse Gas Capture via Halogenation of Metal–Organic Frameworks

Journal of the American Chemical Society Ronald T. Jerozal, Jaehwan Kim, Carolyn Ma et al. Feb 26, 2025 DOI: 10.1021/jacs.5c00393

Self-Assembled Subwavelength Nanophotonic Structures for Spatial Object Localization and Tracking

Journal of the American Chemical Society Jianpeng Ma, Ziguang Zhao, Yingjie Zhao et al. Feb 26, 2025 DOI: 10.1021/jacs.4c14899

The Role of Interfaces and Charge for Chemical Reactivity in Microdroplets

Journal of the American Chemical Society R. Allen LaCour, Joseph P. Heindel, Ruoqi Zhao et al. Feb 26, 2025 DOI: 10.1021/jacs.4c15493

Chemical Synthesis Reveals Pathogenic Role of <i>N</i>-Glycosylation in Microtubule-Associated Protein Tau

Journal of the American Chemical Society Wyatt C. Powell, Ruiheng Jing, Morgane Herlory et al. Feb 26, 2025 DOI: 10.1021/jacs.4c17873

Optimization, application effects and improved microecology of a composite microbial agent containing oyster shells

Scientific Reports Ya-Ting Yang, Xin-Peng Li, Li-Cheng Gao et al. Feb 26, 2025 DOI: 10.1038/s41598-025-91165-y

Three-Coordinate Iron(0) Complex-Catalyzed Regioselective C–H Alkylation of Indole Derivatives

Journal of the American Chemical Society Zi-Jing Zhang, Stéphane Golling, Silvia Cattani et al. Feb 26, 2025 DOI: 10.1021/jacs.4c17316

The effect of cysteine oxidation on conformational changes of SARS-CoV-2 spike protein using atomistic simulations

Scientific Reports Maryam Ghasemitarei, Hoda Taeb, Tayebeh Ghorbi et al. Feb 26, 2025 DOI: 10.1038/s41598-025-90918-z

Recombination of Autodissociated Water Ions in a Nanoscale Pure Water Droplet

Journal of the American Chemical Society Soonho Kwon, Prabhat Prakash, Yixiang Cao et al. Feb 26, 2025 DOI: 10.1021/jacs.4c15103

Early detection of feline chronic kidney disease via 3-hydroxykynurenine and machine learning

Scientific Reports Ellen Vanden Broecke, Laurens Van Mulders, Ellen De Paepe et al. Feb 26, 2025 DOI: 10.1038/s41598-025-90019-x

Enabling Thermally Stimulated Delayed Phosphorescence in Cu(I) Cyclic Trinuclear Complexes with Near-Unity Quantum Yield

Journal of the American Chemical Society Guo-Quan Huang, Ri-Qin Xia, Xu Chen et al. Feb 26, 2025 DOI: 10.1021/jacs.4c09907

Study on energy-autonomous technology for energy consumption performance and climate adaptation in independent public toilets based on DesignBuilder simulation

Scientific Reports Dapeng Bi, Zhonghua Zhao, Qunwu Huang et al. Feb 26, 2025 DOI: 10.1038/s41598-025-91215-5

If your heart stops, this smartwatch-AI can call for help

Nature Benjamin Thompson, Nick Petrić Howe Feb 26, 2025 DOI: 10.1038/d41586-025-00601-6

Copper-Catalyzed Selective Amino-alkoxycarbonylation of Unactivated Alkenes with CO

Journal of the American Chemical Society Si-Shun Yan, Ralf Jackstell, Matthias Beller Feb 26, 2025 DOI: 10.1021/jacs.4c13723