Quasi-homoepitaxy of hexagonal boron nitride on its own interfacial insertion monolayer

P Peng Shen M Maowei Yang Y Yiwei Duo (Research and Development Center for Wide Bandgap Semiconductors, Institute of Semiconductors, Chinese Academy of Sciences 1 , Beijing 100083,) S Shini Yang (Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,) L Lucheng Yu (Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,) Y Yaxiao Lou (Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,) Z Zekai Hu Y Yimeng Wang (Department of Chemistry) F Feiya Xu (Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,) N Na Gao X Xiaohong Chen S Shengrong Huang (Fujian Polytechnic of Information Technology 4 , Fuzhou 350003,) T Tongbo Wei (Research and Development Center for Wide Bandgap Semiconductors, Institute of Semiconductors, Chinese Academy of Sciences 1 , Beijing 100083,) D Duanjun Cai (Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,) J Junyong Kang (Engineering Research Center of Micro-nano Optoelectronic Materials and Devices, Ministry of Education; Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, and Department of Physics, Xiamen University 1 , Xiamen 361005,)

Abstract

We present an approach to improve the quality of hexagonal boron nitride (hBN) epilayer with a quasi-homoepitaxy mode through the utilization of a hBN interfacial insertion monolayer by using metal-organic chemical vapor deposition. First-principles calculations demonstrate that the insertion of hBN monolayer can not only eliminate the interaction from hetero-substrate but also enhance the surface migration rate during epitaxy. As a result with epitaxial growth, the reduction of initial nucleation density of hBN domains is observed, and meanwhile, the release of misfit stress and higher crystal quality are obtained. Ultimately, this research provides a quasi-homoepitaxial strategy of hBN on arbitrary hetero-substrate.

Article Details

Volume / Issue Vol. 126, Issue 7
Published February 17, 2025
ISSN 0003-6951
Publisher American Institute of Physics

Journal Info

Applied Physics Letters

American Institute of Physics

ISSN: 0003-6951 Physical Sciences

Authors (15)

P

Peng Shen

M

Maowei Yang

Y

Yiwei Duo

Research and Development Center for Wide Bandgap Semiconductors, Institute of Semiconductors, Chinese Academy of Sciences 1 , Beijing 100083,

S

Shini Yang

Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,

L

Lucheng Yu

Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,

Y

Yaxiao Lou

Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,

Z

Zekai Hu

Y

Yimeng Wang

Department of Chemistry

F

Feiya Xu

Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,

N

Na Gao

X

Xiaohong Chen

S

Shengrong Huang

Fujian Polytechnic of Information Technology 4 , Fuzhou 350003,

T

Tongbo Wei

Research and Development Center for Wide Bandgap Semiconductors, Institute of Semiconductors, Chinese Academy of Sciences 1 , Beijing 100083,

D

Duanjun Cai

Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, College of Physical Science and Technology, Xiamen University 1 , Xiamen 361005,

J

Junyong Kang

Engineering Research Center of Micro-nano Optoelectronic Materials and Devices, Ministry of Education; Fujian Key Laboratory of Semiconductor Materials and Applications, CI Center for OSED, and Department of Physics, Xiamen University 1 , Xiamen 361005,