Micro-tip manipulated origami for robust twisted few-layer graphene

R Ruo-Jue Zou (Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University , Changsha 410082,) L Long Deng (Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Feringa Nobel Prize Scientist Joint Research Center, School of Chemistry and Molecular Engineering) S Si-Min Xue (Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University , Changsha 410082,) F Feng-Fei Cai (Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University , Changsha 410082,) L Ling-Hui Tong (Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University 1 , Changsha 410082,) Y Yang Zhang Y Yuan Tian L Li Zhang L Lijie Zhang Z Zhihui Qin L Long-Jing Yin (Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University 1 , Changsha 410082,)

Abstract

Twisted few-layer graphene (tFLG) has emerged as an ideal model system for investigating novel strongly correlated and topological phenomena. However, the experimental construction of tFLG with high structural stability is still challenging. Here, we introduce a highly accessible method for fabricating robust tFLG by polymer micro-tip manipulated origami. Through using a self-prepared polymer micro-tip—which is composed of multiple dimethylpolysiloxane, poly(vinyl chloride), and graphite sheets—to fold graphene layers, we fabricated tFLG with different twist angles (0°–30°) and various layers, including twisted bilayers (1 + 1), twisted double-bilayers (2 + 2), twisted double-trilayers (3 + 3), and thicker layers. Even ABC-stacked tFLG were created, such as twisted ABC/ABC and ABC/ABA graphene coexisting in an ABC-ABA domain wall region. We found that the origami-fabricated tFLG exhibits high stability against thermal and mechanical perturbations including heating and transferring, which could be attributed to its special folding and tearing structures. Moreover, based on the rich types of samples, we revealed twist-angle- and stacking-order-dependent Raman characteristics of tFLG, which are valuable for understanding stacking-modulated phonon spectroscopy. Our experiments provide a simple and efficient approach to construct structurally robust tFLG, paving the way for the study of highly stable twisted van der Waals heterostructures.

Article Details

Volume / Issue Vol. 126, Issue 16
Published April 21, 2025
ISSN 0003-6951
Publisher American Institute of Physics

Journal Info

Applied Physics Letters

American Institute of Physics

ISSN: 0003-6951 Physical Sciences

Authors (11)

R

Ruo-Jue Zou

Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University , Changsha 410082,

L

Long Deng

Key Laboratory for Advanced Materials and Joint International Research Laboratory of Precision Chemistry and Molecular Engineering, Feringa Nobel Prize Scientist Joint Research Center, School of Chemistry and Molecular Engineering

S

Si-Min Xue

Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University , Changsha 410082,

F

Feng-Fei Cai

Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University , Changsha 410082,

L

Ling-Hui Tong

Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University 1 , Changsha 410082,

Y

Yang Zhang

Y

Yuan Tian

L

Li Zhang

L

Lijie Zhang

Z

Zhihui Qin

L

Long-Jing Yin

Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education & Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices, School of Physics and Electronics, Hunan University 1 , Changsha 410082,