High-performance multifunctional solar-blind photodetector based on Gd-doped perovskite rare-earth nickelate heterojunctions

J Jiarui Guo (School of Physics, Harbin Institute of Technology 1 , Harbin 150001,) P Pengbo Zhang (State Key Laboratory of Coordination Chemistry, MOE Key Laboratory of Mesoscopic Chemistry, MOE Key Laboratory of High Performance Polymer Materials and Technology, Jiangsu Key Laboratory of Green Energy Catalysis and Intelligent Chemical Engineering, Suzhou Key Laboratory of Green Intelligent Manufacturing of New Energy Materials and Devices, Tianchang New Materials and Energy Technologies Research Center, Institute of Green Chemistry and Engineering, School of Chemistry and Chemical Engineering) L Lingli Zhang L Lingling Tao Y Yu Sui Q Qiang Fu X Xianjie Wang B Bo Song

Abstract

Solar-blind photodetectors based on wide bandgap semiconductors have attracted great interest in recent years. Perovskite rare-earth nickelates are stable p-type semiconductors with adjustable physical properties that are promising candidates for this application. This paper presents a high-performance multifunctional solar-blind photodetector made of NdxGd1−xNiO3/Nb:SrTiO3 heterojunctions utilizing photovoltaic effects. A high position sensitivity of up to 667.03 mV/mm and a fast relaxation time of 1.75 μs were observed under 266 nm laser irradiation and AM1.5 sunlight. A space optical communication system with solar-blindness was achieved. Additionally, an ultraviolet light image sensing system was developed with this device under a light intensity as low as 0.3 μW/cm2. The fast relaxation time and high position sensitivity of rare-earth nickelates make them a promising candidate for self-powered high-performance multifunctional solar-blind detectors.

Article Details

Volume / Issue Vol. 126, Issue 26
Published June 30, 2025
ISSN 0003-6951
Publisher American Institute of Physics

Journal Info

Applied Physics Letters

American Institute of Physics

ISSN: 0003-6951 Physical Sciences

Authors (8)

J

Jiarui Guo

School of Physics, Harbin Institute of Technology 1 , Harbin 150001,

P

Pengbo Zhang

State Key Laboratory of Coordination Chemistry, MOE Key Laboratory of Mesoscopic Chemistry, MOE Key Laboratory of High Performance Polymer Materials and Technology, Jiangsu Key Laboratory of Green Energy Catalysis and Intelligent Chemical Engineering, Suzhou Key Laboratory of Green Intelligent Manufacturing of New Energy Materials and Devices, Tianchang New Materials and Energy Technologies Research Center, Institute of Green Chemistry and Engineering, School of Chemistry and Chemical Engineering

L

Lingli Zhang

L

Lingling Tao

Y

Yu Sui

Q

Qiang Fu

X

Xianjie Wang

B

Bo Song