A perspective on inelastic light scattering spectroscopy for probing transport of collective acoustic excitations

Abstract

Understanding and manipulating nanoscale energy transport and conversion processes are essential for diverse applications, ranging from thermoelectrics and energy harvesting to thermal management of microelectronics. While it has long been recognized that acoustic and thermal properties in condensed matter are primarily due to microscopic transport of phonons as quasiparticles, probing thermal acoustic excitations particularly at subterahertz remains a challenge primarily due to limitations in experimental techniques with spatiotemporal resolutions pertinent to probing them. Brillouin light scattering (BLS) and its variant, impulsive stimulated scattering (ISS), provide access to these thermal acoustic excitations, enabling measurement of quantities such as acoustic dispersions along with relaxation dynamics occurring in ultrasonic as well as hypersonic frequencies. In this Perspective, we provide a brief overview of the operational principles of BLS and ISS and highlight their applications for probing acoustic, thermal, and magnetic excitations in emerging low-dimensional materials. We conclude by discussing current challenges and future opportunities for advanced material characterization using Brillouin light scattering spectroscopy techniques.