Tunable Bipolar Photothermoelectric Response from Mott Activation for In‐Sensor Image Preprocessing

B Bowen Li (Department of Chemistry, College of Arts and Sciences) N Ning Lin Z Zhaowu Wang (School of Science Hebei University of Technology Tianjin 300401 P. R. China) B Baojie Chen (State Key Laboratory of Terahertz and Millimeter Waves City University of Hong Kong Hong Kong 999077 China) C Changyong Lan X Xiaocui Li Y You Meng (Department of Materials Science and Engineering) W Weijun Wang M Mingqi Ding P Pengshan Xie Y Yuxuan Zhang (College of Chemistry) Z Zenghui Wu D Dengji Li F Fu‐Rong Chen (Department of Materials Science and Engineering City University of Hong Kong Kowloon Hong Kong SAR P. R. China) C Chi Hou Chan Z Zhongrui Wang J Johnny C. Ho (Department of Materials Science and Engineering)

Abstract

Abstract In‐sensor image preprocessing, a subset of edge computing, offers a solution to mitigate frequent analog‐digital conversions and the von Neumann bottleneck in conventional digital hardware. However, an efficient in‐sensor device array with large‐scale integration capability for high‐density and low‐power sensory processing is still lacking and highly desirable. This work introduces an adjustable broadband photothermoelectric detector based on a phase‐change vanadium dioxide thin‐film transistor. This transistor employs a vanadium dioxide/gallium nitride three‐terminal structure with a gate‐tunable phase transition at the gate‐source junctions. This design allows for modulable photothermoelectric responsivities and alteration of the short‐circuit photocurrent's polarities. The devices exhibit linear gate dependence for the broadband photoresponse and linear light‐intensity dependence for both positive and negative photoresponsivities. The device's energy consumption is as low as 8 pJ per spike, which is one order of magnitude lower than that of previous Mott materials‐based in‐sensor preprocessing devices. A wafer‐scale bipolar phototransistor array has also been fabricated by standard micro‐/nano‐fabrication techniques, exhibiting excellent stability and endurance (over 5000 cycles). More importantly, an integrated in‐sensor convolutional network is successfully designed for simultaneous broadband image classification, medical image denoising, and retinal vessel segmentation, delivering exceptional performance and paving the way for future smart edge sensors.

Article Details

Volume / Issue Vol. 37, Issue 27
Published July 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (17)

B

Bowen Li

Department of Chemistry, College of Arts and Sciences

N

Ning Lin

Z

Zhaowu Wang

School of Science Hebei University of Technology Tianjin 300401 P. R. China

B

Baojie Chen

State Key Laboratory of Terahertz and Millimeter Waves City University of Hong Kong Hong Kong 999077 China

C

Changyong Lan

X

Xiaocui Li

Y

You Meng

Department of Materials Science and Engineering

W

Weijun Wang

M

Mingqi Ding

P

Pengshan Xie

Y

Yuxuan Zhang

College of Chemistry

Z

Zenghui Wu

D

Dengji Li

F

Fu‐Rong Chen

Department of Materials Science and Engineering City University of Hong Kong Kowloon Hong Kong SAR P. R. China

C

Chi Hou Chan

Z

Zhongrui Wang

J

Johnny C. Ho

Department of Materials Science and Engineering