Tubular Nanostructures from Large‐Pore 2D Covalent Organic Frameworks

J Joaquín Almarza (POLYMAT University of the Basque Country UPV/EHU Avenida de Tolosa 72 Donostia‐San Sebastián 20018 Spain) I Ian Cardillo‐Zallo (School of Chemistry University of Nottingham University Park Nottingham NG7 2RD UK) K Karol Strutyński (CICECO−Aveiro Institute of Materials, Department of Chemistry) M Marta Martínez‐Abadía (POLYMAT University of the Basque Country UPV/EHU Avenida de Tolosa 72 Donostia‐San Sebastián 20018 Spain) N Natalia M. Padial (Functional Inorganic Materials Team, Instituto de Ciencia Molecular (ICMol)) C Carlos Martí‐Gastaldo (Instituto de Ciencia Molecular Universidad de Valencia Paterna 46980 Spain) M Manuel Melle‐Franco (Department of Chemistry, CICECO‐Aveiro Institute of Materials University of Aveiro Aveiro Portugal) A Andrei N. Khlobystov (School of Chemistry) A Aurelio Mateo‐Alonso (POLYMAT, Department of Applied Chemistry University of Basque Country (EHU) Donostia‐San Sebastián Spain)

Abstract

AbstractThe synthesis of a wavy mesoporous 2D covalent organic framework (COF) with a 6‐nm hexagonal pore lattice (Joa‐COF‐1) is reported. This has been achieved by the synthesis of a terpyrenyl linker of approximately 2.7 nm in length and its subsequent condensation with a 3‐connected non‐planar cata‐hexabenzocoronene. Joa‐COF‐1 exists as non‐covalent tubular domains composed of π‐stacked 4 to 5 pores in 2D COF sections that can be separated by mild sonication, resulting in a family of tubular COF nanostructures that combine a 1D morphology with accessible mesopores.

Article Details

Volume / Issue Vol. 64, Issue 23
Published June 02, 2025
ISSN 1433-7851
Publisher Wiley

Journal Info

Angewandte Chemie International Edition

Wiley

ISSN: 1433-7851 Physical Sciences

Authors (9)

J

Joaquín Almarza

POLYMAT University of the Basque Country UPV/EHU Avenida de Tolosa 72 Donostia‐San Sebastián 20018 Spain

I

Ian Cardillo‐Zallo

School of Chemistry University of Nottingham University Park Nottingham NG7 2RD UK

K

Karol Strutyński

CICECO−Aveiro Institute of Materials, Department of Chemistry

M

Marta Martínez‐Abadía

POLYMAT University of the Basque Country UPV/EHU Avenida de Tolosa 72 Donostia‐San Sebastián 20018 Spain

N

Natalia M. Padial

Functional Inorganic Materials Team, Instituto de Ciencia Molecular (ICMol)

C

Carlos Martí‐Gastaldo

Instituto de Ciencia Molecular Universidad de Valencia Paterna 46980 Spain

M

Manuel Melle‐Franco

Department of Chemistry, CICECO‐Aveiro Institute of Materials University of Aveiro Aveiro Portugal

A

Andrei N. Khlobystov

School of Chemistry

A

Aurelio Mateo‐Alonso

POLYMAT, Department of Applied Chemistry University of Basque Country (EHU) Donostia‐San Sebastián Spain