Tailoring the Magnetic Properties of 2D Metal‐Organic Networks by Harnessing the Coordination Sphere

S Shanmugasibi K. Mathialagan (Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain) S Sofia O. Parreiras (Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain) J José Santos (Departamento De Química Orgánica Facultad De Ciencias Químicas Universidad Complutense Madrid 28040 Spain) C Cristina Martín‐Fuentes (Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain) D Daniel Moreno L Lenka Černa (IMDEA Nanoscience C/ Faraday 9, Campus De Cantoblanco Madrid 28049 Spain) M Maria Tenorio (Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain) B Beatriz Muñiz‐Cano (Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain) K Koen Lauwaet (IMDEA Nanoscience, C/ Faraday 9 Campus De Cantoblanco Madrid Spain) M Manuel Valvidares M Miguel A. Valbuena (Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain) J José I. Urgel (IMDEA Nanoscience) W Wolfgang Kuch (Institut für Experimentalphysik Freie Universität Berlin Berlin 14195 Germany) P Pierluigi Gargiani (Department of Materials ETH Zürich Zürich CH‐8093 Switzerland) R Rodolfo Miranda (IMDEA Nanoscience, C/ Faraday 9 Campus De Cantoblanco Madrid Spain) J José I. Martínez (ESISNA Group, Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC), Sor Juana Inés de la Cruz 3, Madrid 28049, Spain) J José M. Gallego (Instituto De Ciencia de Materiales de Madrid (ICMM) CSIC, Cantoblanco Madrid Spain) N Nazario Martín (IMDEA Nanoscience, C/ Faraday 9 Campus De Cantoblanco Madrid Spain) D David Écija (IMDEA Nanoscience)

Abstract

Abstract Achieving magnetic ordering in low‐dimensional materials remains a key objective in the field of magnetism. Herein, coordination chemistry emerges as a powerful discipline to promote the stabilization of magnetism at the nanoscale. We present a thorough study of exemplary two‐dimensional metal‐organic nanoarchitectures synthesized on a Au(111) substrate, which are rationalized by using surface‐science techniques and theoretical calculations. By tuning the stoichiometry, two distinct phases based on the same molecular linker coordinated with Co atoms are obtained, though featuring a different coordination sphere. Remarkably, our combined experimental and theoretical results suggest that for one phase the Co centers have an out‐of‐plane antiferromagnetic ground state, whereas for the other the Co atoms display in‐plane antiferromagnetism. These results pave new avenues for designing two‐dimensional (2D) metal‐organic magnets and tailoring their inherent magnetic properties.

Article Details

Volume / Issue Vol. 64, Issue 44
Published October 27, 2025
ISSN 1433-7851
Publisher Wiley

Journal Info

Angewandte Chemie International Edition

Wiley

ISSN: 1433-7851 Physical Sciences

Authors (19)

S

Shanmugasibi K. Mathialagan

Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain

S

Sofia O. Parreiras

Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain

J

José Santos

Departamento De Química Orgánica Facultad De Ciencias Químicas Universidad Complutense Madrid 28040 Spain

C

Cristina Martín‐Fuentes

Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain

D

Daniel Moreno

L

Lenka Černa

IMDEA Nanoscience C/ Faraday 9, Campus De Cantoblanco Madrid 28049 Spain

M

Maria Tenorio

Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain

B

Beatriz Muñiz‐Cano

Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain

K

Koen Lauwaet

IMDEA Nanoscience, C/ Faraday 9 Campus De Cantoblanco Madrid Spain

M

Manuel Valvidares

M

Miguel A. Valbuena

Institution Instituto Madrileño de Estudios Avanzados en Nanociencia (IMDEA Nanoscience) Madrid 28049 Spain

J

José I. Urgel

IMDEA Nanoscience

W

Wolfgang Kuch

Institut für Experimentalphysik Freie Universität Berlin Berlin 14195 Germany

P

Pierluigi Gargiani

Department of Materials ETH Zürich Zürich CH‐8093 Switzerland

R

Rodolfo Miranda

IMDEA Nanoscience, C/ Faraday 9 Campus De Cantoblanco Madrid Spain

J

José I. Martínez

ESISNA Group, Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC), Sor Juana Inés de la Cruz 3, Madrid 28049, Spain

J

José M. Gallego

Instituto De Ciencia de Materiales de Madrid (ICMM) CSIC, Cantoblanco Madrid Spain

N

Nazario Martín

IMDEA Nanoscience, C/ Faraday 9 Campus De Cantoblanco Madrid Spain

D

David Écija

IMDEA Nanoscience