Synthetic Active Liquid Crystals Powered by Acoustic Waves

A Andrey Sokolov J Jaideep Katuri (Materials Science Division Argonne National Laboratory 9700 South Cass Avenue Lemont IL 60439 USA) J Juan J. de Pablo (Pritzker School of Molecular Engineering) A Alexey Snezhko (Materials Science Division Argonne National Laboratory 9700 South Cass Avenue Lemont IL 60439 USA)

Abstract

Abstract Active nematic materials combine orientational order with activity at the microscopic level. Current experimental realizations of active nematics include vibrating elongated particles, cell layers, suspensions of elongated bacteria, and a mixture of bio‐filaments with molecular motors. The majority of active nematics are of biological origin. The realization of a fully synthetic active liquid crystal comprised of a lyotropic chromonic liquid crystal energized by ultrasonic waves, is reported. This synthetic active liquid crystal is free from biological degradation and variability, exhibits phenomenology associated with active nematics, and enables precise and rapid activity control over a significantly extended range. It is demonstrated that the energy of the acoustic field is converted into microscopic extensile stresses disrupting long‐range nematic order and giving rise to an undulation instability and proliferation of topological defects. The emergence of unconventional free‐standing persistent vortices in the nematic director field at high activity levels is revealed. The results provide a foundation for the design of externally energized active liquid crystals with stable material properties and tunable topological defect dynamics crucial for the realization of reconfigurable microfluidic systems.

Article Details

Volume / Issue Vol. 37, Issue 19
Published May 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (4)

A

Andrey Sokolov

J

Jaideep Katuri

Materials Science Division Argonne National Laboratory 9700 South Cass Avenue Lemont IL 60439 USA

J

Juan J. de Pablo

Pritzker School of Molecular Engineering

A

Alexey Snezhko

Materials Science Division Argonne National Laboratory 9700 South Cass Avenue Lemont IL 60439 USA