Synergistic Supramolecular Activation and Dynamic Alkalinity Replenishing for Sustainable Recycling of Ester‐Containing Plastics

J Jun‐Yan Li (Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China) X Xuehui Liu W Wenli An (Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China) L Lei Yan (Department of Materials Science and Engineering) Y Yingqi Kong (Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China) A Aiqin Huang (Key Laboratory of Green Chemistry and Technology College of Chemistry Ministry of Education Sichuan University Chengdu China) L Li Hu (State Key Laboratory of Cognitive Science and Mental Health, Institute of Psychology, Chinese Academy of Sciences) S Shumin Li (School of Earth Sciences and Engineering, Guangdong Provincial Key Lab of Geological Processes and Mineral Resources, Sun Yat-sen University) Z Zhishan Su S Shimei Xu (Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China) Y Yu‐Zhong Wang (Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China)

Abstract

ABSTRACT Although alkaline hydrolysis represents a promising strategy for recycling polyester plastics, its practical deployment is hampered by the alkaline paradox: the excessive alkaline solution is required to sustain reaction kinetics, while it leads to severe equipment corrosion and wastewater burdens. Here we demonstrate a solvent‐induced alkaline self‐replenishing strategy that enables efficient recycling of diverse ester‐containing plastics, including thermosets (e.g., unsaturated polyester resin, epoxy resin, vinyl ester resin) and thermoplastics (e.g., PET, PBAT) under remarkably mild conditions. By exploiting the temperature‐dependent solubility of KOH in 1,3‐dimethyl‐2‐imidazolidinone (DMI), we established a dynamic alkaline balance: low solubility at room temperature confines it largely to the solid phase, whereas heating promotes dissolution that replenishes consumed base and prevents kinetic stagnation. Characterization evidence reveals that DMI acts as a molecular co‐activator, forming supramolecular complexes with K + to enhance OH − nucleophilicity and polarize ester bonds simultaneously. This system allows for the easy recovery of KOH via auto‐precipitation upon cooling, ensuring excellent reusability. Our work offers a universal and cost‐efficient dynamic methodological framework for the sustainable recycling of diverse polymer architectures.

Article Details

Volume / Issue Vol. 65, Issue 30
Published July 20, 2026
ISSN 1433-7851
Publisher Wiley

Journal Info

Angewandte Chemie International Edition

Wiley

ISSN: 1433-7851 Physical Sciences

Authors (11)

J

Jun‐Yan Li

Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China

X

Xuehui Liu

W

Wenli An

Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China

L

Lei Yan

Department of Materials Science and Engineering

Y

Yingqi Kong

Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China

A

Aiqin Huang

Key Laboratory of Green Chemistry and Technology College of Chemistry Ministry of Education Sichuan University Chengdu China

L

Li Hu

State Key Laboratory of Cognitive Science and Mental Health, Institute of Psychology, Chinese Academy of Sciences

S

Shumin Li

School of Earth Sciences and Engineering, Guangdong Provincial Key Lab of Geological Processes and Mineral Resources, Sun Yat-sen University

Z

Zhishan Su

S

Shimei Xu

Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China

Y

Yu‐Zhong Wang

Collaborative Innovation Center for Eco‐Friendly and Fire‐Safety Polymeric Materials (MoE) National Key Laboratory of Advanced Polymer Materials Engineering National Engineering Laboratory of Eco‐Friendly Polymeric Materials (Sichuan) College of Chemistry Sichuan University Chengdu China