Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO <sub>2</sub> Cathodes

S Shengming Li (School of Control Science and Engineering) Q Qianyue Feng Q Qingye Li (State Key Laboratory of Bioinspired Interfacial Materials Science Institute of Functional Nano &amp; Soft Materials (FUNSOM) Soochow University Suzhou 215123 P.R. China) Y Yeping Xie (State Key Laboratory of Bioinspired Interfacial Materials Science Institute of Functional Nano &amp; Soft Materials (FUNSOM) Soochow University Suzhou 215123 P.R. China) P Panpan Xu Z Zhao Wang (State Key Laboratory of Bioinspired Interfacial Materials Science, State and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials, Jiangsu Key Laboratory of Advanced Functional Polymer Materials, Suzhou Key Laboratory of Macromolecular Design and Precision Synthesis, College of Chemistry, Chemical Engineering and Materials Science) Q Qiming Sun (Innovation Center for Chemical Science, College of Chemistry, Chemical Engineering and Materials Science, Jiangsu Key Laboratory of Advanced Negative Carbon Technologies) M Muhan Cao (Institute of Functional Nano and Soft Materials (FUNSOM), Jiangsu Key Laboratory of Advanced Negative Carbon Technologies, Soochow University, 199 Ren’ai Road, Suzhou, Jiangsu 215123, China) Q Qiao Zhang J Jinxing Chen (Department of Chemistry)

Abstract

Abstract The escalating production of lithium‐ion batteries and plastics poses critical challenges to environmental integrity and resource sustainability. Here, we report a synergistic co‐recycling strategy for spent lithium cobalt oxide (LCO) cathodes and waste polyethylene (PE), leveraging the catalytic properties of LCO to oxidize PE into high‐value dicarboxylic acids. Through a combination of density functional theory calculations, electron spin resonance, and in situ infrared spectroscopy, we reveal that lithium‐deficient LCO undergoes a spin‐state transition of Co 3+ to a high‐spin state, facilitating the activation of oxygen and the generation of singlet oxygen. This reactive oxygen species drives the selective oxidation of PE via hydrogen atom transfer, achieving dicarboxylic acid yields of up to 77.5 wt%, markedly exceeding previous benchmarks. Validation with real‐world plastic waste and spent batteries underscores the feasibility of this approach, presenting a sustainable paradigm‐shift solution for the efficient management of lithium‐ion batteries and plastic waste in a circular economy.

Article Details

Volume / Issue Vol. 64, Issue 25
Published June 17, 2025
ISSN 1433-7851
Publisher Wiley

Journal Info

Angewandte Chemie International Edition

Wiley

ISSN: 1433-7851 Physical Sciences

Authors (10)

S

Shengming Li

School of Control Science and Engineering

Q

Qianyue Feng

Q

Qingye Li

State Key Laboratory of Bioinspired Interfacial Materials Science Institute of Functional Nano &amp; Soft Materials (FUNSOM) Soochow University Suzhou 215123 P.R. China

Y

Yeping Xie

State Key Laboratory of Bioinspired Interfacial Materials Science Institute of Functional Nano &amp; Soft Materials (FUNSOM) Soochow University Suzhou 215123 P.R. China

P

Panpan Xu

Z

Zhao Wang

State Key Laboratory of Bioinspired Interfacial Materials Science, State and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials, Jiangsu Key Laboratory of Advanced Functional Polymer Materials, Suzhou Key Laboratory of Macromolecular Design and Precision Synthesis, College of Chemistry, Chemical Engineering and Materials Science

Q

Qiming Sun

Innovation Center for Chemical Science, College of Chemistry, Chemical Engineering and Materials Science, Jiangsu Key Laboratory of Advanced Negative Carbon Technologies

M

Muhan Cao

Institute of Functional Nano and Soft Materials (FUNSOM), Jiangsu Key Laboratory of Advanced Negative Carbon Technologies, Soochow University, 199 Ren’ai Road, Suzhou, Jiangsu 215123, China

Q

Qiao Zhang

J

Jinxing Chen

Department of Chemistry