Suppressing Interfacial‐Accelerated Degradation in Perovskite Solar Cells via Supramolecular Co‐Assembly

B Boyang Lu (School of Chemical Science and Technology Yunnan University Kunming Yunnan China) X Xiaopeng Feng Z Zhipeng Shao M Mingyuan Han (Beijing Key Laboratory of Novel Thin‐Film Solar Cells, School of New Energy North China Electric Power University Beijing China) X Xiaofan Du Q Qichao Meng (State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy Qingdao New Energy Shandong Laboratory Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao China) Y Yaliang Han (State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy Qingdao New Energy Shandong Laboratory Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao China) R Rongxiu Liu (State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy Qingdao New Energy Shandong Laboratory Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao China) Z Ziqiang Su (Beijing Key Laboratory of Novel Thin‐Film Solar Cells, School of New Energy North China Electric Power University Beijing China) B Bingqian Zhang (State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology) H Hao Wei (Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education, College of Chemistry & Materials Science) Z Zucheng Wu C Changcheng Cui S Shengren Xia F Fengzhi Jiang (School of Chemical Science and Technology Yunnan University Kunming Yunnan China) G Guanglei Cui (Qingdao Industrial Energy Storage Research Institute, Qingdao Institute of Bioenergy and Bioprocess Technology)

Abstract

ABSTRACT Metal halide perovskites exhibit exceptional optoelectronic properties, but the perovskite/organic hole‐transport layer interface often accelerates device degradation under thermal and illumination stress. Single‐component interlayers are insufficient to prevent this coupled interfacial failure, leading to simultaneous destabilization of both the perovskite absorber and doped Spiro‐OMeTAD. Here, we report a carbazole‐derived supramolecular co‐assembly composed of ammonium‐functionalized (CzPACl) and flexible oligo(ethylene glycol) (CzOEG) monomers that simultaneously passivates the perovskite surface and stabilizes the adjacent Spiro‐OMeTAD layer. The resulting nanosheet interlayer suppresses non‐radiative recombination, mitigates ionic migration, and preserves the concentration of Spiro‐OMeTAD radical cations, enhancing interfacial wettability and mechanical compliance. Perovskite solar cells incorporating this co‐assembled layer achieve a power conversion efficiency (PCE) of 25.8% and retain over 90% of their initial efficiency after 1000 h of continuous illumination or over 80% after 1000 h of aging at 85°C. This work highlights supramolecular co‐assembly as a rational strategy to suppress coupled interfacial degradation pathways, providing a general approach for stabilizing perovskite optoelectronic devices.

Article Details

Volume / Issue Vol. 1, Issue 1
Published July 06, 2026
ISSN 1433-7851
Publisher Wiley

Journal Info

Angewandte Chemie International Edition

Wiley

ISSN: 1433-7851 Physical Sciences

Authors (16)

B

Boyang Lu

School of Chemical Science and Technology Yunnan University Kunming Yunnan China

X

Xiaopeng Feng

Z

Zhipeng Shao

M

Mingyuan Han

Beijing Key Laboratory of Novel Thin‐Film Solar Cells, School of New Energy North China Electric Power University Beijing China

X

Xiaofan Du

Q

Qichao Meng

State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy Qingdao New Energy Shandong Laboratory Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao China

Y

Yaliang Han

State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy Qingdao New Energy Shandong Laboratory Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao China

R

Rongxiu Liu

State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy Qingdao New Energy Shandong Laboratory Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences Qingdao China

Z

Ziqiang Su

Beijing Key Laboratory of Novel Thin‐Film Solar Cells, School of New Energy North China Electric Power University Beijing China

B

Bingqian Zhang

State Key Laboratory of Photoelectric Conversion and Utilization of Solar Energy, Qingdao New Energy Shandong Laboratory, Qingdao Institute of Bioenergy and Bioprocess Technology

H

Hao Wei

Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education, College of Chemistry & Materials Science

Z

Zucheng Wu

C

Changcheng Cui

S

Shengren Xia

F

Fengzhi Jiang

School of Chemical Science and Technology Yunnan University Kunming Yunnan China

G

Guanglei Cui

Qingdao Industrial Energy Storage Research Institute, Qingdao Institute of Bioenergy and Bioprocess Technology