Steering Yolk–Shell Nanostructures of 1D Unit‐Based Covalent Organic Frameworks as Binder Modulators

Y Yiwen Yang (Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering) F Fengxue Duan (Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) State Key Laboratory of High Pressure and Superhard Materials College of Physics Jilin University Changchun 130012 China) X Xiaoman Yao (Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China) Z Zhe Xuan (Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China) X Xuanxu Chen (Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China) M Mingjin Shi (Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University Guangzhou 510006 P.R. China) Z Zhengyang Chen (Guizhou Province Key Laboratory of Metallurgical Engineering and Process Energy Saving, College of Materials and Metallurgy Guizhou University Guiyang Guizhou 550025 China) T Taoping Huang (Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China) Y Yifa Chen Y Ya‐Qian Lan (Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou P. R. China)

Abstract

Abstract Induced by their weak chain interactions, 1D unit‐based covalent organic frameworks (1D COFs) are favorable in molecular assembly, yet their exploration in morphology engineering and related energy storage applications are still rare. Here, a series of 1D COFs based nano‐structures (i.e. yolk–shell spheres (YS‐COF), hollow spheres (HS‐COF) and solid spheres (SS‐COF)) is prepared via a solvent‐induced strategy that can be applied as binder modulators for Li‐S batteries. Specifically, they can impart enhanced mechanical properties, more adaptability to volume change, and better ability in adsorbing/catalyzing lithium polysulfide intermediates (LiPSs) to traditional PVDF binder. Remarkably, the thus‐assembled YS‐COF‐based cell displays an initial specific capacity of up to 1011 mAh g −1 at 0.5 C, which is much higher than that of HS‐COF, SS‐COF, and PVDF‐based Li‐S batteries. Even at 4 C, it still maintains a discharge specific capacity of 962 mAh g −1 and can cycle for >600 cycles. DFT calculations and finite element simulation reveal the important roles of nanomorphology and functional groups of YS‐COF in promoting electrochemical redox kinetics to boost battery performances. This strategy might provide in‐depth insights in the morphology engineering and performance optimization of 1D COFs for Li‐S batteries.

Article Details

Volume / Issue Vol. 37, Issue 30
Published July 01, 2025
ISSN 0935-9648
Publisher Unknown Publisher

Journal Info

Advanced Materials

Unknown Publisher

ISSN: 0935-9648 Physical Sciences

Authors (10)

Y

Yiwen Yang

Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering

F

Fengxue Duan

Key Laboratory of Physics and Technology for Advanced Batteries (Ministry of Education) State Key Laboratory of High Pressure and Superhard Materials College of Physics Jilin University Changchun 130012 China

X

Xiaoman Yao

Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China

Z

Zhe Xuan

Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China

X

Xuanxu Chen

Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China

M

Mingjin Shi

Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization, School of Chemistry South China Normal University Guangzhou 510006 P.R. China

Z

Zhengyang Chen

Guizhou Province Key Laboratory of Metallurgical Engineering and Process Energy Saving, College of Materials and Metallurgy Guizhou University Guiyang Guizhou 550025 China

T

Taoping Huang

Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou 510006 P. R. China

Y

Yifa Chen

Y

Ya‐Qian Lan

Guangdong Provincial Key Laboratory of Carbon Dioxide Resource Utilization School of Chemistry South China Normal University Guangzhou P. R. China