Response surface modeling of oxidized polyethylene drag reduction for hydraulic fracturing

H Haowen Yuan Q Qingli Zhu Z Zhiguo Sun C Chao Kang X Xiaolei Zhang (State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering) T Tao Cheng (Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices, Jiangsu Key Laboratory of Advanced Negative Carbon Technologies)

Abstract

Abstract Hydraulic fracturing operations require precise control of friction-reducer dosage to minimize pumping costs, yet the nonlinear coupling between polymer concentration, flow rate, and drag reduction (DR) efficiency remains difficult to predict quantitatively. To address this gap, the present study develops a predictive Response Surface Methodology (RSM) framework for optimizing the DR performance of oxidized polyethylene (1 MDa) in aqueous fracturing fluids. Using a closed-loop pipe flow system (inner diameter 3 cm, test length 10 m), a central composite design (CCD) was executed over the parameter space of polymer concentration (200–600 ppm) and volumetric flow rate (10–50 L/min) at 20 ± 0.5 °C. The resulting quadratic regression model correlating DR% with the two factors is statistically highly significant ( p  < 0.01, R 2 = 0.985, Adj. R 2 = 0.961). The RSM model predicts an optimum DR% of ~ 69.3% at a polymer concentration of ~ 376 ppm and a flow rate of ~ 33 L/min (Re ≈ 35 000), which is experimentally bracketed by the center-point confirmation run (400 ppm, 30 L/min, measured DR% = 69.0%). Validation experiments confirm a prediction error below 2%, and scale-up analysis via empirical scaling laws projects a DR% of 59% under field-relevant conditions (Re = 100 000, large-diameter pipe). Furthermore, temporal degradation tests reveal that DR performance decays exponentially under continuous circulation (first-order rate constant k = 0.045 min −1 ), declining from 70% to 45% within 20 min. These findings provide a reproducible, data-driven basis for real-time dosage optimization and operational fluid management in hydraulic fracturing.

Article Details

Volume / Issue Vol. 1, Issue 1
Published July 22, 2026
ISSN 2045-2322
Publisher Nature Portfolio

Journal Info

Scientific Reports

Nature Portfolio

ISSN: 2045-2322 Open Access Life Sciences

Authors (6)

H

Haowen Yuan

Q

Qingli Zhu

Z

Zhiguo Sun

C

Chao Kang

X

Xiaolei Zhang

State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering

T

Tao Cheng

Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices, Jiangsu Key Laboratory of Advanced Negative Carbon Technologies