Quantum hierarchical Fokker–Planck equations with U(1) gauge fields: Application to the Aharonov–Bohm ring
Abstract
We investigate a three-dimensional subsystem under a time-dependent U(1) gauge field coupled to rotationally invariant environments. To capture the dynamic behavior of the subsystem under thermal excitations and dissipations, it is imperative to treat the bath in a non-Markovian and nonperturbative manner. This is because quantum noise is constrained by the uncertainty principle, which dictates the relationship between the noise correlation time and the amplitude of the energy fluctuation. To this end, we derive the hierarchical equations of motion (HEOM) incorporating the gauge field, enabling a rigorous investigation of the dynamics of the reduced subsystem. Transforming the HEOM into the Wigner representation yields quantum hierarchical Fokker–Planck equations [U(1)-QHFPE] with U(1) gauge fields. These equations incorporate vector fields into the damping operators while preserving both gauge invariance and rotational symmetry. To demonstrate the pratical use of the formalism, we will use it to study the effects of a heat bath on the Aharonov–Bohm (AB) ring. Our investigation includes simulations of the equilibrium distribution, linear absorption spectra, and AB currents under thermal conditions. Within a rotationally invariant system–bath model, we predict the emergence of a persistent current even in dissipative environments, provided the bath is non-Markovian and the temperature is sufficiently low. We also assessed the validity of the Caldeira–Leggett model in this context.
Article Details
Journal Info
The Journal of Chemical Physics
American Institute of Physics
Authors (3)
Hyeonseok Yang
Department of Chemistry, Graduate School of Science, Kyoto University , Kyoto 606-8502,
Shoki Koyanagi
Department of Chemistry, Graduate School of Science, Kyoto University , Kyoto 606-8502,
Yoshitaka Tanimura
Department of Chemistry, Graduate School of Science, Kyoto University 4 , Kyoto 606-8502,