Phase transitions induced by resonant light: A phenomenological approach

A A. Kudlis (Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,) L L. S. Ricco (Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,) H H. Sigurðsson (Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,) I I. A. Shelykh (Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,)

Abstract

We present a phenomenological framework to describe a subclass of light-induced phase transitions (LIPTs) in condensed matter systems, specifically those mediated by the resonant generation of excitons. Our approach extends the classical Landau theory by introducing dynamic coupling between the system’s order parameter and complex excitonic fields, along with Langevin-type forces that drive the system toward states of minimal free energy. The model is applied in the context of all-optical resonant magnetization switching in two-dimensional magnetic materials, particularly reproducing the experimental findings for reverse magnetization by all-optical means for a monolayer CrI3. Our phenomenological model can be applied to other systems characterized by an order parameter and excitonic fields created through resonant light, offering versatility and potential to guide future experimental and theoretical studies in LIPT phenomena.

Article Details

Volume / Issue Vol. 163, Issue 14
Published October 14, 2025
ISSN 0021-9606
Publisher American Institute of Physics

Journal Info

The Journal of Chemical Physics

American Institute of Physics

ISSN: 0021-9606 Physical Sciences

Authors (4)

A

A. Kudlis

Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,

L

L. S. Ricco

Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,

H

H. Sigurðsson

Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,

I

I. A. Shelykh

Science Institute, University of Iceland 1 , Dunhagi-3, IS-107 Reykjavik,