Nature of Anti‐Dissipative High‐Energy Excited States in Quaterpyridine‐Bridged Ruthenium Complexes

N Noémie Chantry (Université catholique de Louvain (UCLouvain) Institut de la Matière Condensée et des Nanosciences (IMCN) Molecular Chemistry Materials and Catalysis (MOST) Place Louis Pasteur 1, bte L4.01.02 Louvain‐la‐Neuve 1348 Belgium) A Agustina Cotic (Universidad de Buenos Aires Facultad de Ciencias Exactas y Naturales Departamento de Química Inorgánica Analítica y Química Física Pabellón 2, Ciudad Universitaria Buenos Aires C1428EHA Argentina) S Simon De Kreijger (Institut de la Matière Condensée et des Nanosciences (IMCN), Molecular Chemistry, Materials and Catalysis (MOST), UCLouvain, Place Louis Pasteur 1/L4.01.02, B-1348 Louvain-la-Neuve, Belgium) R Riccardo Di Forti (Physical Chemistry I Friedrich‐Alexander‐Universität Erlangen‐Nürnberg (FAU) Egerlandstr. 3 91058 Erlangen Germany) B Benjamin Elias (UCLouvain, Institut de la Matière Condensée et des Nanosciences (IMCN), Molecular Chemistry, Materials and Catalysis (MOST), Place Louis Pasteur 1/L4.01.02, B-1348Louvain-la-Neuve, Belgium) L Ludovic Troian‐Gautier (Université catholique de Louvain (UCLouvain) Institut de la Matière Condensée et des Nanosciences (IMCN) Molecular Chemistry Materials and Catalysis (MOST) Place Louis Pasteur 1, bte L4.01.02 Louvain‐la‐Neuve 1348 Belgium) A Alejandro Cadranel (Physical Chemistry I and Interdisciplinary Center for Molecular Materials, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Egerlandstr. 3, 91058 Erlangen, Germany)

Abstract

Abstract High‐energy excited states with slow rates for internal conversion to the lowest‐energy excited state are prone to be intercepted before they dissipate energy to the medium. In a previous report, oligomeric Ru(II) photosensitizers bearing a bridging 2,2′:5′,3″:6″,2 ‴ –quaterpyridine scaffold showed promising anti‐dissipative behavior in photoinduced electron transfer reactivity. In here, a range of electron accepting and electron donating substituents were incorporated on the ancillary 2,2′‐bipyridine ligands to modulate the excited‐state dynamics. This allowed to unambiguously identify the nature of high‐energy excited states and derive design guidelines for the achievement of anti‐dissipative behavior in oligomeric Ru(II) polypyridines relevant for solar fuels production and photoredox catalysis.

Article Details

Volume / Issue Vol. 64, Issue 33
Published August 11, 2025
ISSN 1433-7851
Publisher Wiley

Journal Info

Angewandte Chemie International Edition

Wiley

ISSN: 1433-7851 Physical Sciences

Authors (7)

N

Noémie Chantry

Université catholique de Louvain (UCLouvain) Institut de la Matière Condensée et des Nanosciences (IMCN) Molecular Chemistry Materials and Catalysis (MOST) Place Louis Pasteur 1, bte L4.01.02 Louvain‐la‐Neuve 1348 Belgium

A

Agustina Cotic

Universidad de Buenos Aires Facultad de Ciencias Exactas y Naturales Departamento de Química Inorgánica Analítica y Química Física Pabellón 2, Ciudad Universitaria Buenos Aires C1428EHA Argentina

S

Simon De Kreijger

Institut de la Matière Condensée et des Nanosciences (IMCN), Molecular Chemistry, Materials and Catalysis (MOST), UCLouvain, Place Louis Pasteur 1/L4.01.02, B-1348 Louvain-la-Neuve, Belgium

R

Riccardo Di Forti

Physical Chemistry I Friedrich‐Alexander‐Universität Erlangen‐Nürnberg (FAU) Egerlandstr. 3 91058 Erlangen Germany

B

Benjamin Elias

UCLouvain, Institut de la Matière Condensée et des Nanosciences (IMCN), Molecular Chemistry, Materials and Catalysis (MOST), Place Louis Pasteur 1/L4.01.02, B-1348Louvain-la-Neuve, Belgium

L

Ludovic Troian‐Gautier

Université catholique de Louvain (UCLouvain) Institut de la Matière Condensée et des Nanosciences (IMCN) Molecular Chemistry Materials and Catalysis (MOST) Place Louis Pasteur 1, bte L4.01.02 Louvain‐la‐Neuve 1348 Belgium

A

Alejandro Cadranel

Physical Chemistry I and Interdisciplinary Center for Molecular Materials, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Egerlandstr. 3, 91058 Erlangen, Germany