Minimizing interference in low-pressure supersonic beam sources

J Jack Kelsall (Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,) A Aleksandar Radić (Department of Physics, Cavendish Laboratory) J John Ellis (Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,) D David J. Ward (Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,) A Andrew P. Jardine (Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,)

Abstract

Free-jet atomic, cluster, and molecular sources are typically used to produce beams of low-energy, neutral particles and find application in a wide array of technologies, from neutral atom microscopes to instruments for surface processing. We present a simple analytical theory that is applicable to many of these sources, when (i) the nozzle-skimmer distance is such that free molecular flow is achieved and (ii) there is negligible interference within the skimmer itself. The utility of the model is demonstrated by comparing experimental data with calculations performed using the theory. In particular, we show that skimmer interference is negligible compared to attenuation by “background” gas for room-temperature beams. Our treatment does not depend on any free parameters and obviates the complexity of previous theories. As a result, we are able to devise a number of design recommendations to minimize interference in sources operating with cryogenic-temperature beams.

Article Details

Volume / Issue Vol. 162, Issue 9
Published March 07, 2025
ISSN 0021-9606
Publisher American Institute of Physics

Journal Info

The Journal of Chemical Physics

American Institute of Physics

ISSN: 0021-9606 Physical Sciences

Authors (5)

J

Jack Kelsall

Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,

A

Aleksandar Radić

Department of Physics, Cavendish Laboratory

J

John Ellis

Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,

D

David J. Ward

Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,

A

Andrew P. Jardine

Cavendish Laboratory, Department of Physics, University of Cambridge , JJ Thomson Avenue, Cambridge,