Influence of nitrogen on coherent longitudinal optical phonons in GaAs1− <i>x</i> N <i>x</i>

H Hideo Takeuchi (Department of Physics and Electronics, Graduate School of Engineering, Osaka Metropolitan University (formerly Osaka City University) 1 , 1-1 Gakuen, Naka, Sakai, Osaka 599-8531,) K Kai Matsunaga (Department of Physics and Electronics, Graduate School of Engineering, Osaka Metropolitan University (formerly Osaka City University) 1 , 1-1 Gakuen, Naka, Sakai, Osaka 599-8531,) Y Yusuke Sengi (Department of Applied Physics, Graduate School of Engineering, Osaka City University (currently Osaka Metropolitan University) 2 , 3-3-138, Sugimoto, Sumiyoshi, Osaka 558-8585,) J Jared W. Mitchell (Department of Physics, University of Michigan 2 , Ann Arbor, Michigan 48109,) Y Yury Turkulets R Rachel S. Goldman (Department of Materials Science and Engineering, University of Michigan 1 , Ann Arbor, Michigan 48109,)

Abstract

We investigated the influence of nitrogen (N) on coherent longitudinal optical (LO) phonons in dilute nitride semiconductor alloys. Terahertz time-domain spectroscopy reveals a reduced frequency (redshift) of LO phonons and enhanced decay times for coherent GaAs-like LO phonons emitted from GaAs1−xNx in comparison to those from semi-insulating GaAs. We attribute the redshift of the phonon frequency to both N-alloying-induced compression of the As-sublattice and tensile coherency strain at the GaAs1−xNx/GaAs interface. In addition, an N-induced enhancement of the coherent phonon decay time is attributed to reduced LO phonon scattering associated with the enhanced electron effective masses that reduce the transient electron velocity.

Article Details

Volume / Issue Vol. 138, Issue 23
Published December 21, 2025
ISSN 0021-8979
Publisher American Institute of Physics

Journal Info

Journal of Applied Physics

American Institute of Physics

ISSN: 0021-8979 Physical Sciences

Authors (6)

H

Hideo Takeuchi

Department of Physics and Electronics, Graduate School of Engineering, Osaka Metropolitan University (formerly Osaka City University) 1 , 1-1 Gakuen, Naka, Sakai, Osaka 599-8531,

K

Kai Matsunaga

Department of Physics and Electronics, Graduate School of Engineering, Osaka Metropolitan University (formerly Osaka City University) 1 , 1-1 Gakuen, Naka, Sakai, Osaka 599-8531,

Y

Yusuke Sengi

Department of Applied Physics, Graduate School of Engineering, Osaka City University (currently Osaka Metropolitan University) 2 , 3-3-138, Sugimoto, Sumiyoshi, Osaka 558-8585,

J

Jared W. Mitchell

Department of Physics, University of Michigan 2 , Ann Arbor, Michigan 48109,

Y

Yury Turkulets

R

Rachel S. Goldman

Department of Materials Science and Engineering, University of Michigan 1 , Ann Arbor, Michigan 48109,