iMOE: prediction of second-life battery degradation trajectory using interpretable mixture of experts
Abstract
Abstract Retired electric vehicle batteries offer immense potential to support energy infrastructure stability in underdeveloped regions through second-life use, but uncertainties in battery degradation behaviors pose major safety concerns. This work proposes an interpretable mixture of experts (iMOE) network that predicts battery degradation trajectories using partial, field-accessible signals in a single cycling operation. iMOE leverages an adaptive multi-degradation prediction module to classify battery degradation modes using expert weight synthesis learned from battery capacity-voltage and relaxation data. The module produces latent degradation trend embeddings, which are input to a use-dependent recurrent network for long-term degradation trajectory prediction. Validated on three typical use patterns (i.e. consistent operating histories, deeply aged batteries with unknown prior use, and uncertain second-life conditions, including 295 batteries, 93 use conditions, and 84,213 cycles), iMOE achieves an average mean absolute percentage errors (MAPE) of 0.95% with a 0.43 ms inference time for life-long battery degradation trajectory prediction. Compared to state-of-the-art Informer and PatchTST, it reduces computational time and MAPE by 50% and 77%, respectively. Compatible with data sampling in random state of charge regions, iMOE supports a 150-cycle time-horizon degradation trajectory prediction with 1.50% and 6.26% MAPE on average and at maximum, respectively. Notably, iMOE can operate effectively even with pruned 5MB training data while retaining 0.95% MAPE. Broadly, this network offers a deployable, history-free solution for battery degradation trajectory prediction at the time of second-life deployment, redefining how second-life energy storage systems are sensed, evaluated, controlled, and integrated for sustainable energy infrastructures at scale.
Article Details
Authors (10)
Xinghao Huang
Shengyu Tao
Chen Liang
MOE Key Laboratory for Non-Equilibrium Synthesis and Modulation of Condensed Matter, School of Physics
Yining Tang
Jiawei Chen
State Key Laboratory of Advanced Materials for Intelligent Sensing and Key Laboratory of Organic Integrated Circuits, Ministry of Education & Tianjin Key Laboratory of Molecular Optoelectronic Sciences, Institute of Molecular Plus, Department of Chemistry
Junzhe Shi
Yuqi Li
Bizhong Xia
Guangmin Zhou
Xuan Zhang