Femtosecond-laser-induced optical confinement with ping-pong motion

K Krishna Kant Singh (Department of Chemistry, Indian Institute of Technology Kanpur , Kanpur,) A Ajitesh Singh (Department of Chemistry, Indian Institute of Technology Kanpur , Kanpur,) D Deepak Kumar D Debabrata Goswami (Department of Chemistry, Indian Institute of Technology Kanpur , Kanpur,)

Abstract

We introduce a novel method using a kilohertz (kHz) amplified 800 nm laser for the first experimental confinement of microparticles within a single beam. This study demonstrates that high-energy kHz pulses can confine 1-μm-radius polystyrene beads in water within ∼26 μm. This approach utilizes the unique properties of high-energy pulsed lasers, distinct from continuous-wave and megahertz pulsed lasers traditionally used in optical trapping. The pulsing nature of the kHz laser generates strong instantaneous forces that attract and confine particles within a specific region, inducing a “ping-pong” motion within the confined space. When the laser pulses strike the microparticles, the strong gradient forces pull the particles toward the laser focus, while the scattering force from the laser pushes them away. This interaction creates a dynamic equilibrium, causing the particles to oscillate continuously in a back-and-forth motion until the laser is blocked. This phenomenon differs from conventional optical trapping, which offers unique particle confinement possibilities. When combined with optical trapping, especially at femtomolar concentrations or single-particle conditions, this novel development shows that the kHz laser draws particles from significant distances toward the focal point, enhancing its trapping efficiency. All experiments were conducted on a single setup, varying only laser characteristics, ensuring high credibility in the results.

Article Details

Volume / Issue Vol. 163, Issue 10
Published September 14, 2025
ISSN 0021-9606
Publisher American Institute of Physics

Journal Info

The Journal of Chemical Physics

American Institute of Physics

ISSN: 0021-9606 Physical Sciences

Authors (4)

K

Krishna Kant Singh

Department of Chemistry, Indian Institute of Technology Kanpur , Kanpur,

A

Ajitesh Singh

Department of Chemistry, Indian Institute of Technology Kanpur , Kanpur,

D

Deepak Kumar

D

Debabrata Goswami

Department of Chemistry, Indian Institute of Technology Kanpur , Kanpur,