Evidence for a metal–bosonic insulator–superconductor transition in compressed sulfur

K Kui Wang (Key Lab of Biomass Energy and Material, Jiangsu Province; Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Institute of Chemical Industry of Forest Products) H Hongjian Zhao (Key Laboratory of Material Simulation Methods and Software of Ministry of Education, College of Physics, Jilin University) G Guangtao Liu (Key Laboratory of Material Simulation Methods & Software of Ministry of Education, College of Physics) M Mi Zhou Y Yinqi Chen (State Key Laboratory of Superhard Materials, College of Physics, Jilin University) Q Qiushi Li (State Key Laboratory of Superhard Materials, College of Physics, Jilin University) G Guangchen Ma (State Key Laboratory of Superhard Materials, College of Physics, Jilin University) H Hongbo Wang (State Key Laboratory of High Pressure and Superhard Materials, College of Physics) R Russell J. Hemley (Department of Physics, University of Illinois Chicago) Y Yanming Ma

Abstract

The abrupt drop of resistance to zero at a critical temperature is a key signature of the current paradigm of the metal–superconductor transition. However, the emergence of an intermediate bosonic insulating state characterized by a resistance peak preceding the onset of the superconducting transition has challenged this traditional understanding. Notably, this phenomenon has been predominantly observed in disordered or chemically doped low-dimensional systems, raising intriguing questions about the generality of the effect and its underlying fundamental physics. Here, we present a systematic experimental study of compressed elemental sulfur, an undoped three-dimensional (3D) high-pressure superconductor, with detailed measurements of electrical resistance as a function of temperature, magnetic field, and current. The anomalous resistance peak observed in this 3D system is interpreted based on an empirical model of a metal–bosonic insulator–superconductor transition, potentially driven by vortex dynamics under magnetic field and energy dissipation processes. These findings offer a fresh platform for theoretical analysis of the decades-long enigmatic of the underlying mechanism of this phenomenon.

Article Details

Volume / Issue Vol. 122, Issue 1
Published January 07, 2025
ISSN 0027-8424
Publisher National Academy of Sciences

Authors (10)

K

Kui Wang

Key Lab of Biomass Energy and Material, Jiangsu Province; Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Institute of Chemical Industry of Forest Products

H

Hongjian Zhao

Key Laboratory of Material Simulation Methods and Software of Ministry of Education, College of Physics, Jilin University

G

Guangtao Liu

Key Laboratory of Material Simulation Methods & Software of Ministry of Education, College of Physics

M

Mi Zhou

Y

Yinqi Chen

State Key Laboratory of Superhard Materials, College of Physics, Jilin University

Q

Qiushi Li

State Key Laboratory of Superhard Materials, College of Physics, Jilin University

G

Guangchen Ma

State Key Laboratory of Superhard Materials, College of Physics, Jilin University

H

Hongbo Wang

State Key Laboratory of High Pressure and Superhard Materials, College of Physics

R

Russell J. Hemley

Department of Physics, University of Illinois Chicago

Y

Yanming Ma