Electron-ion equilibration in superheated gold

T Travis D. Griffin D Dirk O. Gericke D Daniel Haden H Hae Ja Lee E Eric Galtier E Eric Cunningham D Dimitri Khaghani M Michael Larsen L Lennart Wollenweber B Ben Armentrout C Carson Convery K Karen Appel G Gilliss Dyer L Luke B. Fletcher S Sebastian Göde J J. B. Hastings J Jeremy Iratcabal E Emma E. McBride J Jacob Molina G Giulio Monaco L Landon Morrison H Hunter Stramel S Sameen Yunus U Ulf Zastrau S Siegfried H. Glenzer G Gianluca Gregori B Bob Nagler T Thomas G. White

Abstract

Abstract Electron-ion equilibration dynamics in samples driven into superheated states with multi-eV electron temperatures represent a fundamental process in nonequilibrium physics. A clear picture of the evolving ion temperature is essential for understanding the strength of the electron-ion coupling. However, direct, model-independent measurements of the ion temperature in laser-irradiated samples have remained experimentally elusive. Using inelastic X-ray scattering with meV-resolution in gold samples, the ion response to ultrafast heating by the hot electrons can be resolved, quantifying the electron-ion equilibration dynamics. We report measurements revealing a strongly enhanced energy transfer rate compared to that in weakly excited gold. Moreover, we obtain a quasi-constant electron-ion coupling at the highly elevated electron temperatures. These results place new constraints on electron-ion energy transfer in warm dense matter and establish a path toward quantitative benchmarking of models for nonequilibrium dynamics.

Article Details

Volume / Issue Vol. 17, Issue 1
Published June 18, 2026
ISSN 2041-1723
Publisher Nature Portfolio

Journal Info

Nature Communications

Nature Portfolio

ISSN: 2041-1723 Open Access Life Sciences

Authors (28)

T

Travis D. Griffin

D

Dirk O. Gericke

D

Daniel Haden

H

Hae Ja Lee

E

Eric Galtier

E

Eric Cunningham

D

Dimitri Khaghani

M

Michael Larsen

L

Lennart Wollenweber

B

Ben Armentrout

C

Carson Convery

K

Karen Appel

G

Gilliss Dyer

L

Luke B. Fletcher

S

Sebastian Göde

J

J. B. Hastings

J

Jeremy Iratcabal

E

Emma E. McBride

J

Jacob Molina

G

Giulio Monaco

L

Landon Morrison

H

Hunter Stramel

S

Sameen Yunus

U

Ulf Zastrau

S

Siegfried H. Glenzer

G

Gianluca Gregori

B

Bob Nagler

T

Thomas G. White