Dissipative quantum geometric phase in the spin-boson system

B Boyu Wang (Center of Single-Molecule Sciences, Institute of Modern Optics, Frontiers Science Center for New Organic Matter, Tianjin Key Laboratory of Micro-scale Optical Information Science and Technology, College of Electronic Information and Optical Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin 300350, P. R. China) M Milan Radonjić (I. Institut für Theoretische Physik, Universität Hamburg 1 , Notkestraße 9, 22607 Hamburg,) F Florian Otterpohl (I. Institut für Theoretische Physik, Universität Hamburg 1 , Notkestraße 9, 22607 Hamburg,) M Michael Thorwart (I. Institut für Theoretische Physik, Universität Hamburg, Notkestr. 9, Hamburg 22607, Germany)

Abstract

We explore how the dissipative geometric phase evolves within the spin-boson model, focusing specifically on coupling to an Ohmic bath in the weakly coherent regime. To determine the non-unitary time evolution of the system’s reduced density matrix, we employ the non-interacting blip approximation (NIBA). For the localized pure initial state used throughout, we derive a compact Bloch-sphere expression showing that the mixed-state geometric phase is a weighted azimuthal winding of the dissipative trajectory. We then map geometric-phase accumulation across various system–bath coupling strengths, temperatures, static biases, and bath cutoff frequencies. Benchmarking representative results against the numerically exact time-evolving matrix product operator (TEMPO) technique shows that NIBA reproduces the population dynamics almost indistinguishably. It also captures the geometric phase quantitatively and qualitatively, although TEMPO reveals a clearer trend in the stationary coherence. Our results show that quantum dissipation suppresses the geometric phase through two complementary mechanisms: thermal noise reduces the state’s purity, while static bias localizes the dynamics and reduces the accessible geometric area.

Article Details

Volume / Issue Vol. 164, Issue 22
Published June 14, 2026
ISSN 0021-9606
Publisher American Institute of Physics

Journal Info

The Journal of Chemical Physics

American Institute of Physics

ISSN: 0021-9606 Physical Sciences

Authors (4)

B

Boyu Wang

Center of Single-Molecule Sciences, Institute of Modern Optics, Frontiers Science Center for New Organic Matter, Tianjin Key Laboratory of Micro-scale Optical Information Science and Technology, College of Electronic Information and Optical Engineering, Nankai University, 38 Tongyan Road, Jinnan District, Tianjin 300350, P. R. China

M

Milan Radonjić

I. Institut für Theoretische Physik, Universität Hamburg 1 , Notkestraße 9, 22607 Hamburg,

F

Florian Otterpohl

I. Institut für Theoretische Physik, Universität Hamburg 1 , Notkestraße 9, 22607 Hamburg,

M

Michael Thorwart

I. Institut für Theoretische Physik, Universität Hamburg, Notkestr. 9, Hamburg 22607, Germany