Comprehensive analysis of effect of high-acid-value waste cooking oil on adhesion between aged asphalt and aggregates

Z Zhiyu Wang (College of New Materials and New Energies) Q Qiang Pei K Kunjie Li Z Zhonghui Wang X Xiaodong Huo Y Yongwei Wang Y Yanfang Li (Shanxi Key Laboratory of Coal-based Value-added Chemicals Green Catalysis Synthesis, School of Chemistry and Chemical Engineering) S Shaoqi Kong

Abstract

Waste cooking oil (WCO) has widespread applications in the rejuvenation of aged asphalt. A few investigations have been conducted on the multiscale adhesion properties and rejuvenation mechanism of aged asphalt-aggregate surfaces treated with high-acid-value WCO. This research focuses on the implications of WCO on the interfacial adhesion of aged asphalt from both macroscopic and microscopic structural viewpoints. The asphalt–aggregate interfacial adhesion was macroscopically assessed through binder bond strength (BBS) tests, and the microscopic mechanism of activation was investigated using a molecular dynamics model. The findings show that through promoting microstructure recovery and mitigating the adverse consequences of aging, WCO might enhance the adhesion strength of aged asphalt. Although the effects of aging on asphalt interface adhesive depend on mineral category, WCO could enhance adhesion along with moisture resistance over the aged asphalt-aggregate boundary. Furthermore, binding strength and interface adhesion work have a strong positive association. This research provides an exhaustive knowledge of the adhesive characteristics of the asphalt-aggregate interface at the multiscale level.

Article Details

Journal PLoS ONE
Volume / Issue Vol. 20, Issue 11
Published November 12, 2025
Pages e0332738
ISSN 1932-6203
Publisher Public Library of Science

Journal Info

PLoS ONE

Public Library of Science

ISSN: 1932-6203 Open Access Health Sciences

Authors (8)

Z

Zhiyu Wang

College of New Materials and New Energies

Q

Qiang Pei

K

Kunjie Li

Z

Zhonghui Wang

X

Xiaodong Huo

Y

Yongwei Wang

Y

Yanfang Li

Shanxi Key Laboratory of Coal-based Value-added Chemicals Green Catalysis Synthesis, School of Chemistry and Chemical Engineering

S

Shaoqi Kong