Bayesian inference of anisotropic 2D small-angle scattering from sparse measurement

C Chi-Huan Tung (Neutron Scattering Division, Oak Ridge National Laboratory 1 , Oak Ridge, Tennessee 37831,) Y Yangyang Wang (Wuya College of Innovation) J Jan-Michael Carrillo (Center for Nanophase Materials Sciences, Oak Ridge National Laboratory 3 , Oak Ridge, Tennessee 37831,) Y Yuya Shinohara (Materials Science and Technology Division, Oak Ridge National Laboratory 6 , Oak Ridge, Tennessee 37831,) C Chun-Yu Chen J Jhih-Min Lin (National Synchrotron Radiation Research Center 4 , 101 Hsin Ann Rd., Hsinchu City 300,) L Lionel Porcar (Institut Laue-Langevin) R Ryan P. Murphy (NIST Center for Neutron Research, National Institute of Standards and Technology 6 , Gaithersburg, Maryland 20878,) G Guan-Rong Huang (Department of Engineering and System Science, National Tsing Hua University 2 , Hsinchu 30013,) L Lijie Ding (Xi’an Jiaotong University , , , ,) C Changwoo Do (Neutron Scattering Division) W Wei-Ren Chen (Neutron Scattering Division, Oak Ridge National Laboratory 1 , Oak Ridge, Tennessee 37831,)

Abstract

We present a Bayesian inference framework for reconstructing anisotropic two-dimensional small-angle scattering (2D SAS) patterns from sparse, noisy, or partially missing data. The method combines a symmetry-aware angular basis with radial Gaussian process priors to enable accurate, training-free interpolation and denoising. Computational benchmarks demonstrate reliable recovery of both isotropic and high-order anisotropic features under severe data reduction. Experimental validations on stretched polymers, sheared wormlike micelles, and carbon fibers show improved fidelity and resolution compared to raw measurements, achieving comparable accuracy with up to 50-fold fewer detected neutrons. This approach enables quantitative structural analysis under low-flux, time-limited, or single-shot conditions, extending the applicability of 2D SAS techniques to compact neutron sources and mechanically driven soft matter systems undergoing transient structural changes.

Article Details

Volume / Issue Vol. 163, Issue 15
Published October 21, 2025
ISSN 0021-9606
Publisher American Institute of Physics

Journal Info

The Journal of Chemical Physics

American Institute of Physics

ISSN: 0021-9606 Physical Sciences

Authors (12)

C

Chi-Huan Tung

Neutron Scattering Division, Oak Ridge National Laboratory 1 , Oak Ridge, Tennessee 37831,

Y

Yangyang Wang

Wuya College of Innovation

J

Jan-Michael Carrillo

Center for Nanophase Materials Sciences, Oak Ridge National Laboratory 3 , Oak Ridge, Tennessee 37831,

Y

Yuya Shinohara

Materials Science and Technology Division, Oak Ridge National Laboratory 6 , Oak Ridge, Tennessee 37831,

C

Chun-Yu Chen

J

Jhih-Min Lin

National Synchrotron Radiation Research Center 4 , 101 Hsin Ann Rd., Hsinchu City 300,

L

Lionel Porcar

Institut Laue-Langevin

R

Ryan P. Murphy

NIST Center for Neutron Research, National Institute of Standards and Technology 6 , Gaithersburg, Maryland 20878,

G

Guan-Rong Huang

Department of Engineering and System Science, National Tsing Hua University 2 , Hsinchu 30013,

L

Lijie Ding

Xi’an Jiaotong University , , , ,

C

Changwoo Do

Neutron Scattering Division

W

Wei-Ren Chen

Neutron Scattering Division, Oak Ridge National Laboratory 1 , Oak Ridge, Tennessee 37831,