Bayesian inference of anisotropic 2D small-angle scattering from sparse measurement
Abstract
We present a Bayesian inference framework for reconstructing anisotropic two-dimensional small-angle scattering (2D SAS) patterns from sparse, noisy, or partially missing data. The method combines a symmetry-aware angular basis with radial Gaussian process priors to enable accurate, training-free interpolation and denoising. Computational benchmarks demonstrate reliable recovery of both isotropic and high-order anisotropic features under severe data reduction. Experimental validations on stretched polymers, sheared wormlike micelles, and carbon fibers show improved fidelity and resolution compared to raw measurements, achieving comparable accuracy with up to 50-fold fewer detected neutrons. This approach enables quantitative structural analysis under low-flux, time-limited, or single-shot conditions, extending the applicability of 2D SAS techniques to compact neutron sources and mechanically driven soft matter systems undergoing transient structural changes.
Article Details
Journal Info
The Journal of Chemical Physics
American Institute of Physics
Authors (12)
Chi-Huan Tung
Neutron Scattering Division, Oak Ridge National Laboratory 1 , Oak Ridge, Tennessee 37831,
Yangyang Wang
Wuya College of Innovation
Jan-Michael Carrillo
Center for Nanophase Materials Sciences, Oak Ridge National Laboratory 3 , Oak Ridge, Tennessee 37831,
Yuya Shinohara
Materials Science and Technology Division, Oak Ridge National Laboratory 6 , Oak Ridge, Tennessee 37831,
Chun-Yu Chen
Jhih-Min Lin
National Synchrotron Radiation Research Center 4 , 101 Hsin Ann Rd., Hsinchu City 300,
Lionel Porcar
Institut Laue-Langevin
Ryan P. Murphy
NIST Center for Neutron Research, National Institute of Standards and Technology 6 , Gaithersburg, Maryland 20878,
Guan-Rong Huang
Department of Engineering and System Science, National Tsing Hua University 2 , Hsinchu 30013,
Lijie Ding
Xi’an Jiaotong University , , , ,
Changwoo Do
Neutron Scattering Division
Wei-Ren Chen
Neutron Scattering Division, Oak Ridge National Laboratory 1 , Oak Ridge, Tennessee 37831,