Anapole enhanced deep-ultraviolet third harmonic generation in a TiO2 metasurface

J Jingyu Wang (Department of Engineering Science, University of Oxford) W Weimin Yang (State Key Laboratory of Green Chemical Engineering and Industrial Catalysis) Y Yonglin He (School of Electronic Information, Zhangzhou Institute of Technology 2 , Zhangzhou 363000,)

Abstract

The deep ultraviolet (DUV) radiation source serves as a critical component in lithography systems, where its energy conversion performance significantly impacts applications in nanoscale photonics and quantum physics. This study presents a theoretical framework achieving exceptional third-harmonic generation with an efficiency higher than 10−2% in the DUV spectrum under optimal conditions and power scaling. Through carefully designed TiO2 nanostructures deposited on metal films, we observe pronounced anapole mode excitation that dramatically amplifies localized field intensities while facilitating nonlinear optical interactions. These findings provide crucial insights into how dielectric nanostructures with moderate refractive indices can manipulate DUV frequency conversion via anapole states, offering new possibilities for developing compact nonlinear optical devices and subwavelength light sources.

Article Details

Volume / Issue Vol. 163, Issue 23
Published December 21, 2025
ISSN 0021-9606
Publisher American Institute of Physics

Journal Info

The Journal of Chemical Physics

American Institute of Physics

ISSN: 0021-9606 Physical Sciences

Authors (3)

J

Jingyu Wang

Department of Engineering Science, University of Oxford

W

Weimin Yang

State Key Laboratory of Green Chemical Engineering and Industrial Catalysis

Y

Yonglin He

School of Electronic Information, Zhangzhou Institute of Technology 2 , Zhangzhou 363000,